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@ARTICLE{Jia:878450,
      author       = {Jia, Wei and Wu, Baohu and Sun, Shengtong and Wu, Peiyi},
      title        = {{I}nterfacially stable {MOF} nanosheet membrane with
                      tailored nanochannels for ultrafast and thermo-responsive
                      nanofiltration},
      journal      = {Nano research},
      volume       = {13},
      issn         = {1998-0000},
      address      = {New York, NY [u.a.]},
      publisher    = {Springer},
      reportid     = {FZJ-2020-02858},
      pages        = {2973-2978},
      year         = {2020},
      abstract     = {Two-dimensional nanosheet membranes with responsive
                      nanochannels are appealing for controlled mass
                      transfer/separation, but limited by everchanging thicknesses
                      arising from unstable interfaces. Herein, an interfacially
                      stable, thermo-responsive nanosheet membrane is assembled
                      from twin-chain stabilized metal-organic framework (MOF)
                      nanosheets, which function via two cyclic amide-bearing
                      polymers, thermo-responsive poly(N-vinyl caprolactam) (PVCL)
                      for adjusting channel size, and non-responsive
                      polyvinylpyrrolidone for supporting constant interlayer
                      distance. Owing to the microporosity of MOF nanosheets and
                      controllable interface wettability, the hybrid membrane
                      demonstrates both superior separation performance and stable
                      thermo-responsiveness. Scattering and correlation
                      spectroscopic analyses further corroborate the respective
                      roles of the two polymers and reveal the microenvironment
                      changes of nanochannels are motivated by the dehydration of
                      PVCL chains.},
      cin          = {JCNS-FRM-II / JCNS-1 / MLZ / JCNS-4},
      ddc          = {660},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106 / I:(DE-588b)4597118-3 /
                      I:(DE-Juel1)JCNS-4-20201012},
      pnm          = {6215 - Soft Matter, Health and Life Sciences (POF3-621) /
                      6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
                      / 6G15 - FRM II / MLZ (POF3-6G15)},
      pid          = {G:(DE-HGF)POF3-6215 / G:(DE-HGF)POF3-6G4 /
                      G:(DE-HGF)POF3-6G15},
      experiment   = {EXP:(DE-MLZ)NOSPEC-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000555405300002},
      doi          = {10.1007/s12274-020-2959-6},
      url          = {https://juser.fz-juelich.de/record/878450},
}