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024 7 _ |a 10.1007/s12274-020-2959-6
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100 1 _ |a Jia, Wei
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245 _ _ |a Interfacially stable MOF nanosheet membrane with tailored nanochannels for ultrafast and thermo-responsive nanofiltration
260 _ _ |a New York, NY [u.a.]
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520 _ _ |a Two-dimensional nanosheet membranes with responsive nanochannels are appealing for controlled mass transfer/separation, but limited by everchanging thicknesses arising from unstable interfaces. Herein, an interfacially stable, thermo-responsive nanosheet membrane is assembled from twin-chain stabilized metal-organic framework (MOF) nanosheets, which function via two cyclic amide-bearing polymers, thermo-responsive poly(N-vinyl caprolactam) (PVCL) for adjusting channel size, and non-responsive polyvinylpyrrolidone for supporting constant interlayer distance. Owing to the microporosity of MOF nanosheets and controllable interface wettability, the hybrid membrane demonstrates both superior separation performance and stable thermo-responsiveness. Scattering and correlation spectroscopic analyses further corroborate the respective roles of the two polymers and reveal the microenvironment changes of nanochannels are motivated by the dehydration of PVCL chains.
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650 1 7 |a Polymers, Soft Nano Particles and Proteins
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700 1 _ |a Wu, Baohu
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700 1 _ |a Sun, Shengtong
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700 1 _ |a Wu, Peiyi
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773 _ _ |a 10.1007/s12274-020-2959-6
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|t Nano research
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|u https://juser.fz-juelich.de/record/878450/files/Jia2020_Article_InterfaciallyStableMOFNanoshee.pdf
856 4 _ |y Published on 2020-08-04. Available in OpenAccess from 2021-08-04.
|u https://juser.fz-juelich.de/record/878450/files/wu_Nano-research-draft-SI.pdf
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