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| Hauptseite > Publikationsdatenbank > Dendrite-tolerant all-solid-state sodium batteries and an important mechanism of metal self-diffusion > print |
| Hauptseite > Publikationsdatenbank > Dendrite-tolerant all-solid-state sodium batteries and an important mechanism of metal self-diffusion > print |
| 001 | 878691 | ||
| 005 | 20240711085552.0 | ||
| 024 | 7 | _ | |a 10.1016/j.jpowsour.2020.228666 |2 doi |
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| 100 | 1 | _ | |a Tsai, Chih-Long |0 P:(DE-Juel1)156244 |b 0 |u fzj |
| 245 | _ | _ | |a Dendrite-tolerant all-solid-state sodium batteries and an important mechanism of metal self-diffusion |
| 260 | _ | _ | |a New York, NY [u.a.] |c 2020 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Inhibition of dendrite growth in all-solid-state lithium batteries (ASSLBs) has long been a challenge to the field.In the present study, the conditions for dendrite growth for a similar but less mature technology, all-solid-statesodium batteries (ASSNBs), are investigated. By simply sticking sodium metal to Na3.4Zr2(SiO4)2.4(PO4)0.6(NZSP) ceramic pellets and without applying external pressure during operation, the critical current density ofNa/NZSP/Na symmetric ASSNBs reaches 9 mA cm 2 at 25 ◦C. The cells can be stably operated at an areal capacityof 5 mAh cm 2 (per half cycle, with 1.0 mA cm 2) at 25 ◦C for 300 h in a galvanostatic cycling measurementwithout any dendrite formation. The results outperform the existing ASSLBs and ASSNBs, and also gobeyond satisfying the requirements for practical applications. The influence of the high metal self-diffusioncoefficient on the dendritic plating/stripping is regarded as the most likely reason for the high dendrite toleranceof ASSNBs. A mathematical model based on Fick’s second law was applied as a first approximation toillustrate this influence. Full ASSNBs were fabricated with infiltrated Na3V2(PO4)3 (NVP) as the cathode and canbe stably operated with a capacity of 0.60 mAh cm 2 at high rate of 0.5 mA cm 2 at room temperature. |
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| 700 | 1 | _ | |a Dellen, Christian |0 P:(DE-Juel1)158085 |b 2 |u fzj |
| 700 | 1 | _ | |a Ling, Yihan |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Ma, Qianli |0 P:(DE-Juel1)129628 |b 4 |e Corresponding author |
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| 773 | _ | _ | |a 10.1016/j.jpowsour.2020.228666 |g Vol. 476, p. 228666 - |0 PERI:(DE-600)1491915-1 |p 228666 - |t Journal of power sources |v 476 |y 2020 |x 0378-7753 |
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| 856 | 4 | _ | |y Published on 2020-08-18. Available in OpenAccess from 2022-08-18. |u https://juser.fz-juelich.de/record/878691/files/Final%20Draft.pdf |
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