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@ARTICLE{Zeng:878726,
author = {Zeng, Fanlin and Malzbender, Jürgen and Baumann, Stefan
and Krüger, Manja and Winnubst, Louis and Guillon, Olivier
and Meulenberg, Wilhelm A.},
title = {{P}hase and microstructural characterizations for
{C}e0.8{G}d0.2{O}2--{F}e{C}o2{O}4 dual phase oxygen
transport membranes},
journal = {Journal of the European Ceramic Society},
volume = {40},
number = {15},
issn = {0955-2219},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2020-03026},
pages = {5646 - 5652},
year = {2020},
abstract = {Dual phase oxygen transport membranes were prepared via
solid state reaction at 1200 ℃. The sintered membranes
were characterized via X-ray diffraction, back scattered
electron microscopy and electron backscatter diffraction,
and associated with image analysis and calculations to
quantify phase compositions and microstructural features
including volume fractions, grain sizes, and contiguity. The
characterizations reveal a multi-phase system containing
Ce1-xGdxO2-δ’ (x ≈ 0.1) (CGO10), and FeyCo3-yO4 (0.2 <
y < 1.2) (FCO), CoO and Gd0.85Ce0.15Fe0.75Co0.25O3 (GCFCO)
in the sintered membranes. In addition, a novel model is
utilized to assess the evolution of the ambipolar
conductivity with respect to microstructural features. Both
experimental and calculated results indicate that if the
grain sizes of all phases in the composites are similar, the
optimal ambipolar conductivity is reached with a volume
ratio of ionic conducting phase to electronic conducting
phase close to 4:1. Meanwhile, the GCFCO phase dominates the
effective electronic conductivity.},
cin = {IEK-1 / IEK-2 / JARA-ENERGY},
ddc = {660},
cid = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-2-20101013 /
$I:(DE-82)080011_20140620$},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113)},
pid = {G:(DE-HGF)POF3-113},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000564729500001},
doi = {10.1016/j.jeurceramsoc.2020.06.035},
url = {https://juser.fz-juelich.de/record/878726},
}