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@ARTICLE{Li:884067,
author = {Li, Qianyu and Wu, Jinglu and Zhou, Jianchao and Sakiev,
Kadyrbek and Hofmann, Diana},
title = {{O}ccurrence of polycyclic aromatic hydrocarbon ({PAH}) in
soils around two typical lakes in the western {T}ian {S}han
{M}ountains ({K}yrgyzstan, {C}entral {A}sia): {L}ocal burden
or global distillation?},
journal = {Ecological indicators},
volume = {108},
issn = {1470-160X},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2020-03076},
pages = {1-9},
year = {2020},
abstract = {The United Nations Educational, Scientific and Cultural
Organization (UNESCO) world natural heritage Tian Shan
Mountains, situated in Central Asia, have experienced a
dramatic increase in polycyclic aromatic hydrocarbon (PAH)
contamination, not only because of increasing volumes of
tourism-derived traffic but also because of the atmospheric
transport of polluted westerly winds under global
distillation effect. To assess the significance of two
possible sources of PAHs, 16 priority PAHs were determined
in 39 soil samples collected in August 2013 around Lake
Issyk-Kul (YKR, 1,606 m) and Lake Son-Kul (SKR, 3,010 m) as
typical mountain lakes in the western Tian Shan Mountains.
Total PAH concentrations ranged from 52 ng/g dw to 9439 ng/g
dw. The highest PAH levels were found in the industrial and
urban areas of the YKR (>1000 ng/g dw); however higher
levels were in the agricultural and rural areas of two
regions (300-1000 ng/g dw), both dominated by 4-,5-ringed
PAHs. In contrast, the lowest PAH levels (<200 ng/g dw) were
mostly distributed in the pristine areas, dominated by
3-,4-ringed PAHs. Diagnostic ratio and Positive Matrix
Factorization model infer that high PAH levels were mainly
generated by petroleum combustion derived from local
burgeoning tourism traffic beside road construction,
indicated by simultaneously measured n-alkanes features (low
carbon preference index and pristane/phytane ratio close to
1 with high unresolved complex mixture values). On the
contrary, low PAH levels primarily from biomass combustion
with unburned petroleum processes are ascribed to exogenous
atmospheric transport under global distillation effect,
because n-alkane sources here are biogenic input without
petroleum contamination. An altitudinal/temperature
dependence of 2-,3- and 4-ringed PAHs was significant in the
SKR, and the soils in the SKR serve as a “sink” for PAHs
in global cycling.},
cin = {IBG-3},
ddc = {630},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {255 - Terrestrial Systems: From Observation to Prediction
(POF3-255)},
pid = {G:(DE-HGF)POF3-255},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000493902400068},
doi = {10.1016/j.ecolind.2019.105749},
url = {https://juser.fz-juelich.de/record/884067},
}