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@ARTICLE{Mhanna:884092,
      author       = {Mhanna, Ramona and Catrou, Pierre and Dutta, Sujeet and
                      Lefort, Ronan and Essafri, Ilham and Ghoufi, Aziz and
                      Muthmann, Matthias and Zamponi, Michaela and Frick, Bernhard
                      and Morineau, Denis},
      title        = {{D}ynamic {H}eterogeneities in {L}iquid {M}ixtures
                      {C}onfined in {N}anopores},
      journal      = {The journal of physical chemistry / B},
      volume       = {124},
      number       = {15},
      issn         = {1520-5207},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2020-03089},
      pages        = {3152 - 3162},
      year         = {2020},
      abstract     = {Binary liquid mixtures can exhibit nanosegregation, albeit
                      being fully miscible and homogeneous at the macroscopic
                      scale. This tendency can be amplified by geometrical
                      nanoconfinement, leading to remarkable properties. This work
                      investigates the molecular dynamics of tert-butanol
                      (TBA)–toluene (TOL) mixtures confined in silica
                      nanochannels by quasielastic neutron scattering and
                      molecular dynamics simulation. It reveals a decoupling of
                      the molecular motion of each constituent of the binary
                      liquid, which can be followed independently by selective
                      isotopic H/D labeling. We argue that this behavior is the
                      signature of spatially segregated dynamic heterogeneities,
                      which are due to the recently established core–shell
                      nanophase separation induced by mesoporous confinement.},
      cin          = {JCNS-FRM-II / MLZ},
      ddc          = {530},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3},
      pnm          = {6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
                      Neutron Research (JCNS) (POF3-623)},
      pid          = {G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
      experiment   = {EXP:(DE-MLZ)SPHERES-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:32216348},
      UT           = {WOS:000526368900019},
      doi          = {10.1021/acs.jpcb.0c01035},
      url          = {https://juser.fz-juelich.de/record/884092},
}