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@ARTICLE{Pozzer:884240,
author = {Pozzer, Andrea and Schultz, Martin G. and Helmig, Detlev},
title = {{I}mpact of {U}.{S}. {O}il and {N}atural {G}as {E}mission
{I}ncreases on {S}urface {O}zone {I}s {M}ost {P}ronounced in
the {C}entral {U}nited {S}tates},
journal = {Environmental science $\&$ technology},
volume = {54},
number = {19},
issn = {0013-936X},
address = {Columbus, Ohio},
publisher = {American Chemical Society},
reportid = {FZJ-2020-03139},
pages = {12423–12433},
year = {2020},
abstract = {Observations of volatile organic compounds (VOCs) from a
surface sampling network and simulation results from the
EMAC (ECHAM5/MESSy for Atmospheric Chemistry) model were
analyzed to assess the impact of increased emissions of VOCs
and nitrogen oxides from U.S. oil and natural gas $(O\&NG)$
sources on air quality. In the first step, the VOC
observations were used to optimize the magnitude and
distribution of atmospheric ethane and higher-alkane VOC
emissions in the model inventory for the base year 2009.
Observation-based increases of the emissions of VOCs and NOx
stemming from U.S. oil and natural gas $(O\&NG)$ sources
during 2009–2014 were then added to the model, and a set
of sensitivity runs was conducted for assessing the
influence of the increased emissions on summer surface ozone
levels. For the year 2014, the added $O\&NG$ emissions are
predicted to affect surface ozone across a large
geographical scale in the United States. These emissions are
responsible for an increased number of days when the
averaged 8-h ozone values exceed 70 ppb, with the highest
sensitivity being in the central and midwestern United
States, where most of the $O\&NG$ growth has occurred. These
findings demonstrate that $O\&NG$ emissions significantly
affect the air quality across most of the United States, can
regionally offset reductions of ozone precursor emissions
made in other sectors, and can have a determining influence
on a region’s ability to meet National Ambient Air Quality
Standard (NAAQS) obligations for ozone.},
cin = {JSC},
ddc = {333.7},
cid = {I:(DE-Juel1)JSC-20090406},
pnm = {512 - Data-Intensive Science and Federated Computing
(POF3-512) / Earth System Data Exploration (ESDE)},
pid = {G:(DE-HGF)POF3-512 / G:(DE-Juel-1)ESDE},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:32902267},
UT = {WOS:000580444600080},
doi = {10.1021/acs.est.9b06983},
url = {https://juser.fz-juelich.de/record/884240},
}