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@ARTICLE{Barnett:884796,
author = {Barnett, Julian and Rose, Marc‐André and Ulrich, Georg
and Lewin, Martin and Kästner, Bernd and Hoehl, Arne and
Dittmann, Regina and Gunkel, Felix and Taubner, Thomas},
title = {{P}honon‐{E}nhanced {N}ear‐{F}ield {S}pectroscopy to
{E}xtract the {L}ocal {E}lectronic {P}roperties of {B}uried
2{D} {E}lectron {S}ystems in {O}xide {H}eterostructures},
journal = {Advanced functional materials},
volume = {30},
number = {46},
issn = {1616-3028},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2020-03258},
pages = {2004767},
year = {2020},
abstract = {In the family of functional oxide materials, the interface
between LaAlO3 and SrTiO3 (LAO/STO) is an interesting
example, as both materials are large‐bandgap insulators in
their bulk state but give rise to a confined 2D electron gas
(2DEG) when combined through thin‐film deposition. While
this 2DEG exhibits remarkable properties, its experimental
investigation is mostly limited to destructive or
non‐local (i.e. averaging over larger areas) methods until
recently. Scanning near‐field optical microscopy is shown
to overcome this limitation, detecting buried 2DEGs by using
highly confined optical near‐fields. Here, a full
spectroscopic approach with phonon‐enhancement and
simulations based on the finite dipole model is combined to
extract quantitative electronic properties of the
interfacial LAO/STO 2DEG. This threefold improvement
compared to previous work will enable the quantitative
nanoscale, non‐destructive, sub‐surface analysis of
complex oxide thin films and interfaces, as well as similar
heterostructures.},
cin = {PGI-7 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$},
pnm = {524 - Controlling Collective States (POF3-524)},
pid = {G:(DE-HGF)POF3-524},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000567443000001},
doi = {10.1002/adfm.202004767},
url = {https://juser.fz-juelich.de/record/884796},
}