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@ARTICLE{Rupp:885494,
author = {Rupp, J. A. J. and Janod, E. and Besland, M.-P. and
Corraze, B. and Kindsmüller, A. and Querré, M. and
Tranchant, J. and Cario, L. and Dittmann, R. and Waser, R.
and Wouters, D. J.},
title = {{C}ompetition between {V}2{O}3 phases deposited by one-step
reactive sputtering process on polycrystalline conducting
electrode},
journal = {Thin solid films},
volume = {705},
issn = {0040-6090},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2020-03875},
pages = {138063 -},
year = {2020},
abstract = {This comprehensive work investigates a technologically
appealing synthesis of V2O3 oxide thin films for electronic
applications by the use of direct reactive sputtering with a
heavily diluted gas mixture on a conducting platinum
electrode. Morphological characterization was performed by
Scanning Electron Microscopy, Atomic Force Microscopy, X-Ray
Diffraction and X-Ray Reflectometry. Vanadium valence states
were investigated by X-Ray Photoelectron Spectroscopy and
crystalline phases were checked by X-Ray Grazing Incidence
measurements. Low temperature electrical transport
characteristics were determined by 2-point probe
measurements. Only amorphous V2O3 was found to exist in a
mixed-valence phase in the investigated parameter range.
Deposition temperatures between 400 °C and 550 °C enable
formation of mixtures between crystallographic phases of
corundum- and bixbyite-type V2O3 polymorphs. Depending on
temperature and sputtering power, morphology and
stoichiometry can be tuned to generate four distinct type of
electrical transport characteristics. Most promising
electrical properties of corundum V2O3 with a resistance
ratio of up to four orders of magnitude (during the low
temperature insulator-to-metal transition) have been
obtained for a moderate sputtering power of 50 W (on a 1″
target) at a deposition temperature of 600 °C. Reactive
sputtering thus enables direct control of structural and
electrical parameters for polycrystalline V2O3 thin film
phases on a conducting substrate.},
cin = {PGI-7 / JARA-FIT},
ddc = {660},
cid = {I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$},
pnm = {524 - Controlling Collective States (POF3-524)},
pid = {G:(DE-HGF)POF3-524},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000533601500004},
doi = {10.1016/j.tsf.2020.138063},
url = {https://juser.fz-juelich.de/record/885494},
}