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@ARTICLE{Kerkmann:885496,
author = {Kerkmann, Abhilasha and Schneller, T. and Valov, I. and
Singh, I. B. and Srivastava, A. K. and Waser, R.},
title = {{C}opper facilitated nickel oxy-hydroxide films as
efficient synergistic oxygen evolution electrocatalyst},
journal = {Journal of catalysis},
volume = {384},
issn = {0021-9517},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2020-03877},
pages = {189 - 198},
year = {2020},
abstract = {Efficient catalysts made of cheap and abundant metal ions
are in need to overcome the sluggish kinetics of the anodic
water oxidation reaction. The development of an inexpensive
catalyst with improved performance is key to produce
hydrogen by the electrolytic water splitting reaction. The
user friendly chemical solution deposition method was
applied to prepare films with predecided mole concentrations
of copper and nickel. The mixed metal oxide with equal mole
ratio of Cu:Ni (1:1) achieved the maximum activity with the
onset of water oxidation at overpotential of 0.40 V (1.63 V
vs RHE) and achieved the current density of 1 mA/cm2 at an
overpotential of 0.420 V at pH 13. The activity of this
combination is attributed to the copper facilitated in-situ
formation of a layered nickel oxy-hydroxide structure. The
presence of both metal ions was found to be necessary
indicating a synergy between Cu and Ni for the oxygen
evolution reaction. The present work representing the simple
synthesis process of the catalyst with the improved water
oxidation activity is a promising step to develop electrodes
for water electrolysis.},
cin = {PGI-7 / JARA-FIT / IBI-7},
ddc = {540},
cid = {I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$ /
I:(DE-Juel1)IBI-7-20200312},
pnm = {524 - Controlling Collective States (POF3-524)},
pid = {G:(DE-HGF)POF3-524},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000525490600018},
doi = {10.1016/j.jcat.2020.02.023},
url = {https://juser.fz-juelich.de/record/885496},
}