000885675 001__ 885675
000885675 005__ 20240712112825.0
000885675 0247_ $$2doi$$a10.1021/acsami.0c07523
000885675 0247_ $$2ISSN$$a1944-8244
000885675 0247_ $$2ISSN$$a1944-8252
000885675 0247_ $$2Handle$$a2128/25914
000885675 0247_ $$2altmetric$$aaltmetric:87225208
000885675 0247_ $$2pmid$$apmid:32687702
000885675 0247_ $$2WOS$$aWOS:000563074900024
000885675 037__ $$aFZJ-2020-04006
000885675 041__ $$aEnglish
000885675 082__ $$a600
000885675 1001_ $$0P:(DE-Juel1)161141$$aYu, Shicheng$$b0$$eCorresponding author$$ufzj
000885675 245__ $$aA flexible all–solid–state Li–ion battery manufacturable in ambient atmosphere
000885675 260__ $$aWashington, DC$$bSoc.$$c2020
000885675 3367_ $$2DRIVER$$aarticle
000885675 3367_ $$2DataCite$$aOutput Types/Journal article
000885675 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1602857014_16786
000885675 3367_ $$2BibTeX$$aARTICLE
000885675 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000885675 3367_ $$00$$2EndNote$$aJournal Article
000885675 520__ $$aThe rational design and exploration of safe, robust, and inexpensive energy storage systems with high flexibility are greatly desired for integrated wearable electronic devices. Herein, a flexible all-solid-state battery possessing competitive electrochemical performance and mechanical stability has been realized by easy manufacture processes using carbon nanotube enhanced phosphate electrodes of LiTi2(PO4)3 and Li3V2(PO4)3 and a highly conductive solid polymer electrolyte made of polyphosphazene/PVDF-HFP/LiBOB [PVDF-HFP, poly(vinylidene fluoride-co-hexafluoropropylene)]. The components were chosen based on their low toxicity, systematic manufacturability, and (electro-)chemical matching in order to ensure ambient atmosphere battery assembly and to reach high flexibility, good safety, effective interfacial contacts, and high chemical and mechanical stability for the battery while in operation. The high energy density of the electrodes was enabled by a novel design of the self-standing anode and cathode in a way that a large amount of active particles are embedded in the carbon nanotube (CNT) bunches and on the surface of CNT fabric, without binder additive, additional carbon, or a large metallic current collector. The electrodes showed outstanding performance individually in half-cells with liquid and polymer electrolyte, respectively. The prepared flexible all-solid-state battery exhibited good rate capability, and more than half of its theoretical capacity can be delivered even at 1C at 30 °C. Moreover, the capacity retentions are higher than 75% after 200 cycles at different current rates, and the battery showed smaller capacity fading after cycling at 50 °C. Furthermore, the promising practical possibilities of the battery concept and fabrication method were demonstrated by a prototype laminated flexible cell.
000885675 536__ $$0G:(DE-HGF)POF3-131$$a131 - Electrochemical Storage (POF3-131)$$cPOF3-131$$fPOF III$$x0
000885675 588__ $$aDataset connected to CrossRef
000885675 7001_ $$0P:(DE-Juel1)177996$$aXu, Qi$$b1$$ufzj
000885675 7001_ $$0P:(DE-Juel1)156244$$aTsai, Chih-Long$$b2$$ufzj
000885675 7001_ $$0P:(DE-HGF)0$$aHoffmeyer, Marija$$b3
000885675 7001_ $$0P:(DE-Juel1)176785$$aWiemhöfer, Hans-Dieter$$b4$$ufzj
000885675 773__ $$0PERI:(DE-600)2467494-1$$a10.1021/acsami.0c07523$$gVol. 12, no. 33, p. 37067 - 37078$$n33$$p37067 - 37078$$tACS applied materials & interfaces$$v12$$x1944-8252$$y2020
000885675 8564_ $$uhttps://juser.fz-juelich.de/record/885675/files/acsami.0c07523-1.pdf$$yRestricted
000885675 8564_ $$uhttps://juser.fz-juelich.de/record/885675/files/acsami.0c07523-1.pdf?subformat=pdfa$$xpdfa$$yRestricted
000885675 8564_ $$uhttps://juser.fz-juelich.de/record/885675/files/am-2020-07523n.R1_Proof_hi.pdf$$yPublished on 2020-07-20. Available in OpenAccess from 2021-07-20.
000885675 909CO $$ooai:juser.fz-juelich.de:885675$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000885675 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)161141$$aForschungszentrum Jülich$$b0$$kFZJ
000885675 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)177996$$aForschungszentrum Jülich$$b1$$kFZJ
000885675 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)156244$$aForschungszentrum Jülich$$b2$$kFZJ
000885675 9101_ $$0I:(DE-HGF)0$$6P:(DE-HGF)0$$a Westfälische Wilhelms-Universität Münster$$b3
000885675 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)176785$$aForschungszentrum Jülich$$b4$$kFZJ
000885675 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)176785$$a Westfälische Wilhelms-Universität Münster$$b4
000885675 9131_ $$0G:(DE-HGF)POF3-131$$1G:(DE-HGF)POF3-130$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lSpeicher und vernetzte Infrastrukturen$$vElectrochemical Storage$$x0
000885675 9141_ $$y2020
000885675 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0530$$2StatID$$aEmbargoed OpenAccess
000885675 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)9905$$2StatID$$aIF >= 5$$bACS APPL MATER INTER : 2018$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bACS APPL MATER INTER : 2018$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0310$$2StatID$$aDBCoverage$$bNCBI Molecular Biology Database$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2020-01-05
000885675 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2020-01-05
000885675 920__ $$lyes
000885675 9201_ $$0I:(DE-Juel1)IEK-9-20110218$$kIEK-9$$lGrundlagen der Elektrochemie$$x0
000885675 9801_ $$aFullTexts
000885675 980__ $$ajournal
000885675 980__ $$aVDB
000885675 980__ $$aUNRESTRICTED
000885675 980__ $$aI:(DE-Juel1)IEK-9-20110218
000885675 981__ $$aI:(DE-Juel1)IET-1-20110218