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@ARTICLE{Yu:885675,
      author       = {Yu, Shicheng and Xu, Qi and Tsai, Chih-Long and Hoffmeyer,
                      Marija and Wiemhöfer, Hans-Dieter},
      title        = {{A} flexible all–solid–state {L}i–ion battery
                      manufacturable in ambient atmosphere},
      journal      = {ACS applied materials $\&$ interfaces},
      volume       = {12},
      number       = {33},
      issn         = {1944-8252},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2020-04006},
      pages        = {37067 - 37078},
      year         = {2020},
      abstract     = {The rational design and exploration of safe, robust, and
                      inexpensive energy storage systems with high flexibility are
                      greatly desired for integrated wearable electronic devices.
                      Herein, a flexible all-solid-state battery possessing
                      competitive electrochemical performance and mechanical
                      stability has been realized by easy manufacture processes
                      using carbon nanotube enhanced phosphate electrodes of
                      LiTi2(PO4)3 and Li3V2(PO4)3 and a highly conductive solid
                      polymer electrolyte made of polyphosphazene/PVDF-HFP/LiBOB
                      [PVDF-HFP, poly(vinylidene
                      fluoride-co-hexafluoropropylene)]. The components were
                      chosen based on their low toxicity, systematic
                      manufacturability, and (electro-)chemical matching in order
                      to ensure ambient atmosphere battery assembly and to reach
                      high flexibility, good safety, effective interfacial
                      contacts, and high chemical and mechanical stability for the
                      battery while in operation. The high energy density of the
                      electrodes was enabled by a novel design of the
                      self-standing anode and cathode in a way that a large amount
                      of active particles are embedded in the carbon nanotube
                      (CNT) bunches and on the surface of CNT fabric, without
                      binder additive, additional carbon, or a large metallic
                      current collector. The electrodes showed outstanding
                      performance individually in half-cells with liquid and
                      polymer electrolyte, respectively. The prepared flexible
                      all-solid-state battery exhibited good rate capability, and
                      more than half of its theoretical capacity can be delivered
                      even at 1C at 30 °C. Moreover, the capacity retentions are
                      higher than $75\%$ after 200 cycles at different current
                      rates, and the battery showed smaller capacity fading after
                      cycling at 50 °C. Furthermore, the promising practical
                      possibilities of the battery concept and fabrication method
                      were demonstrated by a prototype laminated flexible cell.},
      cin          = {IEK-9},
      ddc          = {600},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:32687702},
      UT           = {WOS:000563074900024},
      doi          = {10.1021/acsami.0c07523},
      url          = {https://juser.fz-juelich.de/record/885675},
}