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000885886 245__ $$aDNA Self-Assembly Mediated by Programmable Soft-Patchy Interactions
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000885886 520__ $$aAdding shape and interaction anisotropy to a colloidal particle offers exquisitely tunable routes to engineer a rich assortment of complex-architected structures. Inspired by the hierarchical self-assembly concept with block copolymers and DNA liquid crystals and exploiting the unique assembly properties of DNA, we report here the construction and self-assembly of DNA-based soft-patchy anisotropic particles with a high degree of modularity in the system’s design. By programmable positioning of thermoresponsive polymeric patches on the backbone of a stiff DNA duplex with linear and star-shaped architecture, we reversibly drive the DNA from a disordered ensemble to a diverse array of long-range ordered multidimensional nanostructures with tunable lattice spacing, ranging from lamellar to bicontinuous double-gyroid and double-diamond cubic morphologies, through the alteration of temperature. Our results demonstrate that the proposed hierarchical self-assembly strategy can be applied to any kind of DNA nanoarchitecture, highlighting the design principles for integration of self-assembly concepts from the physics of liquid crystals, block copolymers, and patchy colloids into the continuously growing interdisciplinary research field of structural DNA nanotechnology.
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000885886 7001_ $$0P:(DE-HGF)0$$aZhang, Jing$$b1
000885886 7001_ $$0P:(DE-Juel1)130754$$aKentzinger, Emmanuel$$b2
000885886 7001_ $$0P:(DE-Juel1)130928$$aRücker, Ulrich$$b3
000885886 7001_ $$00000-0002-4903-3159$$aPortale, Giuseppe$$b4
000885886 7001_ $$0P:(DE-HGF)0$$aJung, Niklas$$b5
000885886 7001_ $$00000-0002-2161-4541$$aJonas, Ulrich$$b6
000885886 7001_ $$0P:(DE-Juel1)151224$$aMyung, Jin S.$$b7
000885886 7001_ $$0P:(DE-Juel1)131039$$aWinkler, Roland G.$$b8
000885886 7001_ $$0P:(DE-Juel1)130665$$aGompper, Gerhard$$b9
000885886 7001_ $$0P:(DE-Juel1)130616$$aDhont, Jan K. G.$$b10
000885886 7001_ $$0P:(DE-Juel1)130987$$aStiakakis, Emmanuel$$b11$$eCorresponding author$$ufzj
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000885886 8564_ $$uhttps://juser.fz-juelich.de/record/885886/files/Novak_Supporting_Information.pdf$$yPublished on 2020-10-13. Available in OpenAccess from 2021-10-13.
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