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@ARTICLE{Novak:885886,
author = {Novak, Sanja and Zhang, Jing and Kentzinger, Emmanuel and
Rücker, Ulrich and Portale, Giuseppe and Jung, Niklas and
Jonas, Ulrich and Myung, Jin S. and Winkler, Roland G. and
Gompper, Gerhard and Dhont, Jan K. G. and Stiakakis,
Emmanuel},
title = {{DNA} {S}elf-{A}ssembly {M}ediated by {P}rogrammable
{S}oft-{P}atchy {I}nteractions},
journal = {ACS nano},
volume = {14},
number = {10},
issn = {1936-086X},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2020-04162},
pages = {13524–13535},
year = {2020},
abstract = {Adding shape and interaction anisotropy to a colloidal
particle offers exquisitely tunable routes to engineer a
rich assortment of complex-architected structures. Inspired
by the hierarchical self-assembly concept with block
copolymers and DNA liquid crystals and exploiting the unique
assembly properties of DNA, we report here the construction
and self-assembly of DNA-based soft-patchy anisotropic
particles with a high degree of modularity in the system’s
design. By programmable positioning of thermoresponsive
polymeric patches on the backbone of a stiff DNA duplex with
linear and star-shaped architecture, we reversibly drive the
DNA from a disordered ensemble to a diverse array of
long-range ordered multidimensional nanostructures with
tunable lattice spacing, ranging from lamellar to
bicontinuous double-gyroid and double-diamond cubic
morphologies, through the alteration of temperature. Our
results demonstrate that the proposed hierarchical
self-assembly strategy can be applied to any kind of DNA
nanoarchitecture, highlighting the design principles for
integration of self-assembly concepts from the physics of
liquid crystals, block copolymers, and patchy colloids into
the continuously growing interdisciplinary research field of
structural DNA nanotechnology.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / IAS-2 / IBI-4 / IBI-5},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)IAS-2-20090406 /
I:(DE-Juel1)IBI-4-20200312 / I:(DE-Juel1)IBI-5-20200312},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623) / 551 - Functional Macromolecules
and Complexes (POF3-551)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-551},
typ = {PUB:(DE-HGF)16},
pubmed = {33048544},
UT = {WOS:000586793400100},
doi = {10.1021/acsnano.0c05536},
url = {https://juser.fz-juelich.de/record/885886},
}