Hauptseite > Publikationsdatenbank > DNA Self-Assembly Mediated by Programmable Soft-Patchy Interactions > print |
001 | 885886 | ||
005 | 20250129094303.0 | ||
024 | 7 | _ | |a 10.1021/acsnano.0c05536 |2 doi |
024 | 7 | _ | |a 1936-0851 |2 ISSN |
024 | 7 | _ | |a 1936-086X |2 ISSN |
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100 | 1 | _ | |a Novak, Sanja |0 P:(DE-Juel1)167259 |b 0 |
245 | _ | _ | |a DNA Self-Assembly Mediated by Programmable Soft-Patchy Interactions |
260 | _ | _ | |a Washington, DC |c 2020 |b Soc. |
336 | 7 | _ | |a article |2 DRIVER |
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520 | _ | _ | |a Adding shape and interaction anisotropy to a colloidal particle offers exquisitely tunable routes to engineer a rich assortment of complex-architected structures. Inspired by the hierarchical self-assembly concept with block copolymers and DNA liquid crystals and exploiting the unique assembly properties of DNA, we report here the construction and self-assembly of DNA-based soft-patchy anisotropic particles with a high degree of modularity in the system’s design. By programmable positioning of thermoresponsive polymeric patches on the backbone of a stiff DNA duplex with linear and star-shaped architecture, we reversibly drive the DNA from a disordered ensemble to a diverse array of long-range ordered multidimensional nanostructures with tunable lattice spacing, ranging from lamellar to bicontinuous double-gyroid and double-diamond cubic morphologies, through the alteration of temperature. Our results demonstrate that the proposed hierarchical self-assembly strategy can be applied to any kind of DNA nanoarchitecture, highlighting the design principles for integration of self-assembly concepts from the physics of liquid crystals, block copolymers, and patchy colloids into the continuously growing interdisciplinary research field of structural DNA nanotechnology. |
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856 | 4 | _ | |y Published on 2020-10-13. Available in OpenAccess from 2021-10-13. |u https://juser.fz-juelich.de/record/885886/files/Novak_Supporting_Information.pdf |
856 | 4 | _ | |y Published on 2020-10-13. Available in OpenAccess from 2021-10-13. |u https://juser.fz-juelich.de/record/885886/files/Novak_manuscript.pdf |
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