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@ARTICLE{Rok:885912,
author = {Rok, Magdalena and Moskwa, Marcin and Dopieralski,
Przemysław and Medycki, Wojciech and Zamponi, Michaela and
Bator, Grażyna},
title = {{T}he influence of structure on the methyl group dynamics
of polymorphic complexes: 6,6′-dimethyl-2,2′-dipyridyl
with halo derivatives of benzoquinone acids},
journal = {CrystEngComm},
volume = {22},
number = {41},
issn = {1466-8033},
address = {London},
publisher = {RSC},
reportid = {FZJ-2020-04176},
pages = {6811 - 6821},
year = {2020},
note = {template des Verlags!},
abstract = {Recently, interest in organic ferroelectrics or
antiferroelectrics representing a metal-free perovskite-type
has increased significantly. This interest results from the
properties of organic systems. First of all, they do not
have toxic metals in their structure. Therefore they are
environmentally friendly. Also, the method of preparation,
simple syntheses, and low-temperature processability
increase their attractiveness in terms of application. In
this paper, the above properties are associated with the
proton dynamics in organic donor–acceptor systems. We
present the comparison of the physicochemical properties of
four molecular complexes containing the proton acceptor
molecule, 6,6′-dimethyl-2,2′-bipyridyl (66DMBP), and one
of three organic acid molecules belonging to the
benzoquinone group. As proton donor molecules the organic
acids: chloranilic, bromanilic and iodanilic acids have been
chosen. We present the results of experiments concerning the
determination of crystal structures, 1H NMR, inelastic
neutron scattering (INS) and UV/vis spectra. In the
theoretical part, we attempt to explain the influence of the
crystallization method (a type of solvent) on transoid or
cisoid arrangement of 66DMBP. In the theoretical approach,
we focus on two forms of the complex with chloranilic acid,
α-66DMBP·CLA and β-66DMBP·CLA, which undergo
solid-to-solid phase transitions, at 380 and 317 K,
respectively. We have chosen these examples because the α
analogue possesses ferroelectric properties in a wide range
of temperatures.},
cin = {JCNS-FRM-II / JCNS-1 / MLZ},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106 / I:(DE-588b)4597118-3},
pnm = {6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
Neutron Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)SPHERES-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000583363700007},
doi = {10.1039/D0CE00973C},
url = {https://juser.fz-juelich.de/record/885912},
}