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@ARTICLE{Beck:886066,
author = {Beck, Jürgen and Heymann, William and von Lieres, Eric and
Hahn, Rainer},
title = {{C}ompartment {M}odel of {M}ixing in a {B}ubble {T}rap and
{I}ts {I}mpact on {C}hromatographic {S}eparations},
journal = {Processes},
volume = {8},
number = {7},
issn = {2227-9717},
address = {Basel},
publisher = {MDPI},
reportid = {FZJ-2020-04253},
pages = {780 -},
year = {2020},
abstract = {Chromatography equipment includes hold-up volumes that are
external to the packed bed and usually not considered in the
development of chromatography models. These volumes can
substantially contribute to band-broadening in the system
and deteriorate the predicted performance. We selected a
bubble trap of a pilot scale chromatography system as an
example for a hold-up volume with a non-standard mixing
behavior. In a worst-case scenario, the bubble trap is not
properly flushed before elution, thus causing the
significant band-broadening of the elution peak. We showed
that the mixing of buffers with different densities in the
bubble trap device can be accurately modeled using a simple
compartment model. The model was calibrated at a wide range
of flow rates and salt concentrations. The simulations were
performed using the open-source software CADET, and all
scripts and data are published with this manuscript. The
results illustrate the importance of including external
holdup volumes in chromatography modeling. The
band-broadening effect of tubing, pumps, valves, detectors,
frits, or any other zones with non-standard mixing behavior
can be considered in very similar way},
cin = {IBG-1},
ddc = {570},
cid = {I:(DE-Juel1)IBG-1-20101118},
pnm = {583 - Innovative Synergisms (POF3-583)},
pid = {G:(DE-HGF)POF3-583},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000557505800001},
doi = {10.3390/pr8070780},
url = {https://juser.fz-juelich.de/record/886066},
}