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@ARTICLE{Kulyk:886123,
author = {Kulyk, Nadiia and Berger, Daniel and Smith, Ana-Sunčana
and Harting, Jens},
title = {{C}atalytic flow with a coupled finite difference —
{L}attice {B}oltzmann scheme},
journal = {Computer physics communications},
volume = {256},
issn = {0010-4655},
address = {Amsterdam},
publisher = {North Holland Publ. Co.},
reportid = {FZJ-2020-04286},
pages = {107443 -},
year = {2020},
abstract = {Many catalyst devices employ flow through porous
structures, which leads to a complex macroscopic mass and
heat transport. To unravel the detailed dynamics of the
reactive gas flow, we present an all-encompassing model,
consisting of thermal lattice Boltzmann model by Kang et
al., used to solve the heat and mass transport in the gas
domain, coupled to a finite differences solver for the heat
equation in the solid via thermal reactive boundary
conditions for a consistent treatment of the reaction
enthalpy. The chemical surface reactions are incorporated in
a flexible fashion through flux boundary conditions at the
gas–solid interface. We scrutinize the thermal FD-LBM by
benchmarking the macroscopic transport in the gas domain as
well as conservation of the enthalpy across the solid–gas
interface. We exemplify the applicability of our model by
simulating the reactive gas flow through a microporous
material catalyzing the so-called water-gas-shift reaction.},
cin = {IEK-11},
ddc = {530},
cid = {I:(DE-Juel1)IEK-11-20140314},
pnm = {121 - Solar cells of the next generation (POF3-121) / DFG
project 416229255 - SFB 1411: Produktgestaltung disperser
Systeme},
pid = {G:(DE-HGF)POF3-121 / G:(GEPRIS)416229255},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000590251400013},
doi = {10.1016/j.cpc.2020.107443},
url = {https://juser.fz-juelich.de/record/886123},
}