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@ARTICLE{Peixoto:888146,
author = {Peixoto, Thiago R. F. and Bentmann, Hendrik and Rüßmann,
Philipp and Tcakaev, Abdul-Vakhab and Winnerlein, Martin and
Schreyeck, Steffen and Schatz, Sonja and Vidal, Raphael
Crespo and Stier, Fabian and Zabolotnyy, Volodymyr and
Green, Robert J. and Min, Chul Hee and Fornari, Celso I. and
Maaß, Henriette and Vasili, Hari Babu and Gargiani,
Pierluigi and Valvidares, Manuel and Barla, Alessandro and
Buck, Jens and Hoesch, Moritz and Diekmann, Florian and
Rohlf, Sebastian and Kalläne, Matthias and Rossnagel, Kai
and Gould, Charles and Brunner, Karl and Blügel, Stefan and
Hinkov, Vladimir and Molenkamp, Laurens W. and Reinert,
Friedrich},
title = {{N}on-local effect of impurity states on the exchange
coupling mechanism in magnetic topological insulators},
journal = {npj quantum materials},
volume = {5},
number = {1},
issn = {2397-4648},
address = {[London]},
publisher = {Nature Publishing Group},
reportid = {FZJ-2020-04720},
pages = {87},
year = {2020},
abstract = {Since the discovery of the quantum anomalous Hall (QAH)
effect in the magnetically doped topological insulators
(MTI) Cr:(Bi,Sb)2Te3 and V:(Bi,Sb)2Te3, the search for the
magnetic coupling mechanisms underlying the onset of
ferromagnetism has been a central issue, and a variety of
different scenarios have been put forward. By combining
resonant photoemission, X-ray magnetic circular dichroism
and density functional theory, we determine the local
electronic and magnetic configurations of V and Cr
impurities in (Bi,Sb)2Te3. State-of-the-art first-principles
calculations find pronounced differences in their 3d
densities of states, and show how these impurity states
mediate characteristic short-range pd exchange interactions,
whose strength sensitively varies with the position of the
3d states relative to the Fermi level. Measurements on films
with varying host stoichiometry support this trend. Our
results explain, in an unified picture, the origins of the
observed magnetic properties, and establish the essential
role of impurity-state-mediated exchange interactions in the
magnetism of MTI.},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000590981700001},
doi = {10.1038/s41535-020-00288-0},
url = {https://juser.fz-juelich.de/record/888146},
}