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000888204 245__ $$aSignatures of an atomic crystal in the band structure of a C 60 thin film
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000888204 520__ $$aTransport phenomena in molecular materials are intrinsically linked to the orbital character and the degree of localization of the valence states. Here we combine angle-resolved photoemission with photoemission tomography to determine the spatial distribution of all molecular states of the valence band structure of a C60 thin film. While the two most frontier valence states exhibit a strong band dispersion, the states at larger binding energies are characterized by distinct emission patterns in energy and momentum space. Our findings demonstrate the formation of an atomic crystal-like band structure in a molecular solid with delocalized π-like valence states and strongly localized σ states at larger binding energies.
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000888204 7001_ $$0P:(DE-HGF)0$$aLüftner, Daniel$$b1
000888204 7001_ $$0P:(DE-HGF)0$$aHaag, Florian$$b2
000888204 7001_ $$0P:(DE-HGF)0$$aSeidel, Johannes$$b3
000888204 7001_ $$00000-0003-1588-6310$$aKelly, Leah L.$$b4
000888204 7001_ $$0P:(DE-Juel1)162281$$aZamborlini, Giovanni$$b5
000888204 7001_ $$0P:(DE-Juel1)169309$$aJugovac, Matteo$$b6
000888204 7001_ $$0P:(DE-Juel1)145012$$aFeyer, Vitaliy$$b7
000888204 7001_ $$0P:(DE-HGF)0$$aAeschlimann, Martin$$b8
000888204 7001_ $$0P:(DE-HGF)0$$aPuschnig, Peter$$b9
000888204 7001_ $$00000-0003-0735-8921$$aCinchetti, Mirko$$b10
000888204 7001_ $$0P:(DE-Juel1)139025$$aStadtmüller, Benjamin$$b11$$eCorresponding author
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