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000888205 1001_ $$00000-0002-7735-1322$$aLu, Chun-I$$b0
000888205 245__ $$aSpontaneously induced magnetic anisotropy in an ultrathin Co/MoS 2 heterojunction
000888205 260__ $$aCambridge$$bRoyal Society of Chemistry$$c2020
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000888205 520__ $$aMagnetic anisotropy (MA) is a material preference that involves magnetization aligned along a specific direction and provides a basis for spintronic devices. Here we report the first observation of strong MA in a cobalt–molybdenum disulfide (Co/MoS2) heterojunction. Element-specific magnetic images recorded with an X-ray photoemission electron microscope (PEEM) reveal that ultrathin Co films, of thickness 5 monolayers (ML) and above, form micrometer (μm)-sized domains on monolayer MoS2 flakes of size tens of μm. Image analysis shows that the magnetization of these Co domains is oriented not randomly but in directions apparently correlated with the crystal structure of the underlying MoS2. Evidence from micro-area X-ray photoelectron spectra (μ-XPS) further indicates that a small amount of charge is donated from cobalt to sulfur upon direct contact between Co and MoS2. As the ferromagnetic behavior found for Co/MoS2 is in sharp contrast with that reported earlier for non-reactive Fe/MoS2, we suggest that orbital hybridization at the interface is what makes Co/MoS2 different. Our report provides micro-magnetic and micro-spectral evidence that consolidates the knowledge required to build functional heterojunctions based on two-dimensional (2D) materia
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000888205 7001_ $$0P:(DE-HGF)0$$aHuang, Chih-Heng$$b1
000888205 7001_ $$0P:(DE-HGF)0$$aOu Yang, Kui-Hon$$b2
000888205 7001_ $$00000-0001-9102-5876$$aSimbulan, Kristan Bryan$$b3
000888205 7001_ $$0P:(DE-HGF)0$$aLi, Kai-Shin$$b4
000888205 7001_ $$0P:(DE-Juel1)171643$$aLi, Feng$$b5
000888205 7001_ $$00000-0002-1733-7641$$aQi, Junjie$$b6
000888205 7001_ $$0P:(DE-Juel1)169309$$aJugovac, Matteo$$b7
000888205 7001_ $$0P:(DE-Juel1)176932$$aCojocariu, Iulia$$b8
000888205 7001_ $$0P:(DE-Juel1)145012$$aFeyer, Vitaliy$$b9
000888205 7001_ $$0P:(DE-Juel1)168293$$aTusche, Christian$$b10
000888205 7001_ $$0P:(DE-HGF)0$$aLin, Minn-Tsong$$b11
000888205 7001_ $$0P:(DE-HGF)0$$aChuang, Tzu-Hung$$b12
000888205 7001_ $$00000-0003-2403-1357$$aLan, Yann-Wen$$b13$$eCorresponding author
000888205 7001_ $$00000-0002-6877-602X$$aWei, Der-Hsin$$b14$$eCorresponding author
000888205 773__ $$0PERI:(DE-600)2840770-2$$a10.1039/D0NH00108B$$gVol. 5, no. 7, p. 1058 - 1064$$n7$$p1058 - 1064$$tNanoscale horizons$$v5$$x2055-6764$$y2020
000888205 8564_ $$uhttps://juser.fz-juelich.de/record/888205/files/d0nh00108b.pdf
000888205 8564_ $$uhttps://juser.fz-juelich.de/record/888205/files/manuscript.pdf$$yPublished on 2020-04-29. Available in OpenAccess from 2021-04-29.
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