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| Hauptseite > Publikationsdatenbank > Magnetoelectric coupling in the mixed erythrosiderite [(NH$_4$)$_{1−x}$K$_x$]$_2$[FeCl$_5$(H$_2$O)] > print |
| Hauptseite > Publikationsdatenbank > Magnetoelectric coupling in the mixed erythrosiderite [(NH$_4$)$_{1−x}$K$_x$]$_2$[FeCl$_5$(H$_2$O)] > print |
| 001 | 888331 | ||
| 005 | 20230426083224.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevB.102.054413 |2 doi |
| 024 | 7 | _ | |a 0163-1829 |2 ISSN |
| 024 | 7 | _ | |a 0556-2805 |2 ISSN |
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| 024 | 7 | _ | |a 1098-0121 |2 ISSN |
| 024 | 7 | _ | |a 1538-4446 |2 ISSN |
| 024 | 7 | _ | |a 1538-4489 |2 ISSN |
| 024 | 7 | _ | |a 1550-235X |2 ISSN |
| 024 | 7 | _ | |a 2469-9950 |2 ISSN |
| 024 | 7 | _ | |a 2469-9969 |2 ISSN |
| 024 | 7 | _ | |a 2469-9977 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2020-04850 |
| 082 | _ | _ | |a 530 |
| 100 | 1 | _ | |a Brüning, Daniel |0 0000-0001-5830-2683 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Magnetoelectric coupling in the mixed erythrosiderite [(NH$_4$)$_{1−x}$K$_x$]$_2$[FeCl$_5$(H$_2$O)] |
| 260 | _ | _ | |a Woodbury, NY |c 2020 |b Inst. |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1611148473_17121 |2 PUB:(DE-HGF) |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a We present a study of the dielectric, structural and magnetic properties of the multiferroic orlinear magnetoelectric substitution series [(NH4)1xKx]2[FeCl5(H2O)]. Pyroelectric currents, magneticsusceptibilities, and thermodynamic properties were examined on large single crystals of theerythrosiderite compounds and detailed magnetic-eld versus temperature phase diagrams are derivedfor three dierent substitution levels. With increasing potassium concentration the material istuned from a multiferroic (x 0:06) to a linear magnetoelectric (x 0:15) ground state. In contrastto the respective pure parent compounds with x = 0 or 1, however, the ferroelectric or linear magnetoelectricpolarization in none of the substituted samples is switchable by external electric elds,because these samples exhibit a signicant electric polarization already above the magnetic orderingtransition. The polarization arises at a higher-lying structural phase transition that is examined byTHz spectroscopy and by comprehensive neutron-diraction experiments on a deuterated pure singlecrystal. The structural phase transition is attributed to an ordering of NH+4 tetrahedra but doesnot break inversion symmetry in the pure material, while nite K content causes pyroelectricity. |
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| 542 | _ | _ | |i 2020-08-07 |2 Crossref |u https://link.aps.org/licenses/aps-default-license |
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| 700 | 1 | _ | |a Fröhlich, Tobias |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Langenbach, Malte |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Leich, Thomas |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Meven, Martin |0 P:(DE-Juel1)164297 |b 4 |e Corresponding author |
| 700 | 1 | _ | |a Becker, Petra |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Bohatý, Ladislav |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Grüninger, Markus |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Braden, Markus |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Lorenz, Thomas |0 P:(DE-HGF)0 |b 9 |
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| 773 | _ | _ | |a 10.1103/PhysRevB.102.054413 |g Vol. 102, no. 5, p. 054413 |0 PERI:(DE-600)2844160-6 |n 5 |p 054413 |t Physical review / B |v 102 |y 2020 |x 2469-9950 |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/888331/files/PhysRevB.102.054413.pdf |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/888331/files/meven_Paper_NHK-rev_openaccess.pdf |
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