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@ARTICLE{Saha:888372,
      author       = {Saha, Debasish and Peddireddy, Karthik R. and Allgaier, J.
                      and Zhang, Wei and Maccarrone, Simona and Frielinghaus,
                      Henrich and Richter, Dieter},
      title        = {{A}mphiphilic {C}omb {P}olymers as {N}ew {A}dditives in
                      {B}icontinuous {M}icroemulsions},
      journal      = {Nanomaterials},
      volume       = {10},
      number       = {12},
      issn         = {2079-4991},
      address      = {Basel},
      publisher    = {MDPI},
      reportid     = {FZJ-2020-04875},
      pages        = {2410 -},
      year         = {2020},
      abstract     = {It has been shown that the thermodynamics of bicontinuous
                      microemulsions can be tailored via the addition of various
                      different amphiphilic polymers. In this manuscript, we now
                      focus on comb-type polymers consisting of hydrophobic
                      backbones and hydrophilic side chains. The distinct
                      philicity of the backbone and side chains leads to a
                      well-defined segregation into the oil and water domains
                      respectively, as confirmed by contrast variation small-angle
                      neutron scattering experiments. This polymer–microemulsion
                      structure leads to well-described conformational entropies
                      of the polymer fragments (backbone and side chains) that
                      exert pressure on the membrane, which influences the
                      thermodynamics of the overall microemulsion. In the context
                      of the different polymer architectures that have been
                      studied by our group with regards to their phase diagrams
                      and small-angle neutron scattering, the microemulsion
                      thermodynamics of comb polymers can be described in terms of
                      a superposition of the backbone and side chain fragments.
                      The denser or longer the side chain, the stronger the
                      grafting and the more visible the brush effect of the side
                      chains becomes. Possible applications of the comb polymers
                      as switchable additives are discussed. Finally, a balanced
                      philicity of polymers also motivates transmembrane migration
                      in biological systems of the polymers themselves or of
                      polymer–DNA complexes.},
      cin          = {JCNS-FRM-II / JCNS-1 / JCNS-2 / MLZ},
      ddc          = {540},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106 / I:(DE-Juel1)JCNS-2-20110106 /
                      I:(DE-588b)4597118-3},
      pnm          = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
                      / 6G15 - FRM II / MLZ (POF3-6G15) / 6215 - Soft Matter,
                      Health and Life Sciences (POF3-621)},
      pid          = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15 /
                      G:(DE-HGF)POF3-6215},
      experiment   = {EXP:(DE-MLZ)KWS1-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {33276588},
      UT           = {WOS:000602344300001},
      doi          = {10.3390/nano10122410},
      url          = {https://juser.fz-juelich.de/record/888372},
}