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@ARTICLE{MOYNIHAN:888403,
author = {MOYNIHAN, EOIN and ROST, STEFAN and O'CONNELL, EOGHAN and
RAMASSE, QUENTIN and FRIEDRICH, CHRISTOPH and BANGERT,
URSEL},
title = {{P}lasmons in {M}o{S} 2 studied via experimental and
theoretical correlation of energy loss spectra},
journal = {Journal of microscopy},
volume = {279},
number = {3},
issn = {1365-2818},
address = {Oxford [u.a.]},
publisher = {Wiley-Blackwell},
reportid = {FZJ-2020-04882},
pages = {256 - 264},
year = {2020},
abstract = {This paper takes a fundamental view of the electron energy
loss spectra of monolayer and few layer MoS2. The dielectric
function of monolayer MoS2 is compared to the experimental
spectra to give clear criteria for the nature of different
signals. Kramers–Krönig analysis allows a direct
extraction of the dielectric function from the experimental
data. However this analysis is sensitive to slight changes
in the normalisation step of the data pretreatment. Density
functional theory provides simulations of the dielectric
function for comparison and validation of experimental
findings. Simulated and experimental spectra are compared to
isolate the π and π + σ surface plasmon modes in
monolayer MoS2. Single‐particle excitations obscure the
plasmons in the monolayer spectrum and momentum resolved
measurements give indication of indirect interband
transitions that are excited due to the large convergence
and collection angles used in the experiment.},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
ddc = {570},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143) /
Optoelectronic properties of materials for photovoltaic and
photonic applications $(jpgi10_20191101)$},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143 /
$G:(DE-Juel1)jpgi10_20191101$},
typ = {PUB:(DE-HGF)16},
pubmed = {32400884},
UT = {WOS:000539106700001},
doi = {10.1111/jmi.12900},
url = {https://juser.fz-juelich.de/record/888403},
}