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@ARTICLE{Zhu:888455,
      author       = {Zhu, Guangqi and Qi, Yanling and Liu, Fan and Ma, Shenqian
                      and Xiang, Guolei and Jin, Fengmin and Liu, Zigeng and Wei,
                      Wang},
      title        = {{R}econstructing 1{D} {F}e {S}ingle‐atom {C}atalytic
                      {S}tructure on 2{D} {G}raphene film for {H}igh‐efficiency
                      {O}xygen {R}eduction {R}eaction},
      journal      = {ChemSusChem},
      volume       = {14},
      number       = {3},
      issn         = {1864-564X},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2020-04923},
      pages        = {866-875},
      year         = {2021},
      abstract     = {The ordinary intrinsic activity and disordered distribution
                      of metal sites in zero/one-dimensional (0D/1D) single-atom
                      catalysts (SACs) lead to inferior catalytic efficiency and
                      short-term endurance in the oxygen reduction reaction (ORR),
                      which restricts the large-scale application of
                      hydrogen−oxygen fuel cells and metal−air batteries. To
                      improve the activity of SACs, a mild synthesis method was
                      chosen to conjugate 1D Fe SACs with 2D graphene film (Fe
                      SAC@G) that realized a composite structure with well-ordered
                      atomic-Fe coordination configuration. The product exhibits
                      outstanding ORR electrocatalytic efficiency and stability in
                      0.1 M KOH aqueous solution. DFT-D computational results
                      manifest the intrinsic ORR activity of Fe SAC@G originated
                      from the newly-formed FeN4−O−FeN4 bridge structure with
                      moderate adsorption ability towards ORR intermediates. These
                      findings provide new ways for designing SACs with high
                      activity and long-term stability.},
      cin          = {IEK-9},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {122 - Elektrochemische Energiespeicherung (POF4-122)},
      pid          = {G:(DE-HGF)POF4-122},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {33236522},
      UT           = {WOS:000596585900001},
      doi          = {10.1002/cssc.202002359},
      url          = {https://juser.fz-juelich.de/record/888455},
}