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@ARTICLE{Kerber:888657,
author = {Kerber, Nico and Ksenzov, Dmitriy and Freimuth, Frank and
Capotondi, Flavio and Pedersoli, Emanuele and Lopez-Quintas,
Ignacio and Seng, Boris and Cramer, Joel and Litzius, Kai
and Lacour, Daniel and Zabel, Hartmut and Mokrousov, Yuriy
and Kläui, Mathias and Gutt, Christian},
title = {{F}aster chiral versus collinear magnetic order recovery
after optical excitation revealed by femtosecond {XUV}
scattering},
journal = {Nature Communications},
volume = {11},
number = {1},
issn = {2041-1723},
address = {[London]},
publisher = {Nature Publishing Group UK},
reportid = {FZJ-2020-05099},
pages = {6304},
year = {2020},
abstract = {While chiral spin structures stabilized by
Dzyaloshinskii-Moriya interaction (DMI) are candidates as
novel information carriers, their dynamics on the fs-ps
timescale is little known. Since with the bulk Heisenberg
exchange and the interfacial DMI two distinct exchange
mechanisms are at play, the ultrafast dynamics of the chiral
order needs to be ascertained and compared to the dynamics
of the conventional collinear order. Using an XUV
free-electron laser we determine the fs-ps temporal
evolution of the chiral order in domain walls in a magnetic
thin film sample by an IR pump - X-ray magnetic scattering
probe experiment. Upon demagnetization we observe that the
dichroic (CL-CR) signal connected with the chiral order
correlator mzmx in the domain walls recovers significantly
faster than the (CL + CR) sum signal representing the
average collinear domain magnetization mz2 + mx2. We
explore possible explanations based on spin structure
dynamics and reduced transversal magnetization fluctuations
inside the domain walls and find that the latter can explain
the experimental data leading to different dynamics for
collinear magnetic order and chiral magnetic order.},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
ddc = {500},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) /
Topological transport in real materials from ab initio
$(jiff40_20190501)$},
pid = {G:(DE-HGF)POF3-142 / $G:(DE-Juel1)jiff40_20190501$},
typ = {PUB:(DE-HGF)16},
pubmed = {33298908},
UT = {WOS:000600148800005},
doi = {10.1038/s41467-020-19613-z},
url = {https://juser.fz-juelich.de/record/888657},
}