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@ARTICLE{Jeong:888910,
author = {Jeong, Jaehong and Lenz, Benjamin and Gukasov, Arsen and
Fabrèges, Xavier and Sazonov, Andrew and Hutanu, Vladimir
and Louat, Alex and Bounoua, Dalila and Martins, Cyril and
Biermann, Silke and Brouet, Véronique and Sidis, Yvan and
Bourges, Philippe},
title = {{M}agnetization {D}ensity {D}istribution of {S}r 2 {I}r{O}
4 : {D}eviation from a {L}ocal j eff = 1 / 2 {P}icture},
journal = {Physical review letters},
volume = {125},
number = {9},
issn = {1079-7114},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2020-05315},
pages = {097202},
year = {2020},
abstract = {5d iridium oxides are of huge interest due to the potential
for new quantum states driven by strong spin-orbit coupling.
The strontium iridate Sr2IrO4is particularly in the
spotlight because of the so-called jeff=1/2 state consisting
of a quantum superposition of the three local t2g orbitals
with, in its simplest version, nearly equal populations,
which stabilizes an unconventional Mott insulating state.
Here, we reportan anisotropic and aspherical magnetization
density distribution measured by polarized neutron
diffractionin a magnetic field up to 5 T at 4 K, which
strongly deviates from a local jeff=1/2 picture even when
distortion-induced deviations from the equal weights of the
orbital populations are taken into account. Once
reconstructed by the maximum entropy method and multipole
expansion model refinement, the magnetization density shows
four cross-shaped positive lobes along the crystallographic
tetragonal axes with a large spatial extent, showing that
the xy-orbital contribution is dominant.The analogy to the
superconducting copper oxide systems might then be weaker
than commonly thought.},
cin = {JCNS-FRM-II / MLZ},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3},
pnm = {6212 - Quantum Condensed Matter: Magnetism,
Superconductivity (POF3-621) / 6G15 - FRM II / MLZ
(POF3-6G15) / 6G4 - Jülich Centre for Neutron Research
(JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6G15 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)POLI-HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {32915616},
UT = {WOS:000562322000007},
doi = {10.1103/PhysRevLett.125.097202},
url = {https://juser.fz-juelich.de/record/888910},
}