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@ARTICLE{Zobkalo:888916,
author = {Zobkalo, I. A. and Matveeva, A. N. and Sazonov, Andrew and
Barilo, S. N. and Shiryaev, S. V. and Pedersen, Björn and
Hutanu, Vladimir},
title = {{D}irect control of magnetic chirality in {N}d{M} n 2 {O} 5
by external electric field},
journal = {Physical review / B},
volume = {101},
number = {6},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2020-05321},
pages = {064425},
year = {2020},
abstract = {Detailed investigation of the incommensurate magnetic
ordering in a single crystal of multiferroic NdMn2O5 has
been performed using both nonpolarized and polarized
neutron-diffraction techniques. Below TN≈30.5K magnetic
Bragg reflections corresponding to the nonchiral-type
magnetic structure with propagation vector k1=(0.50kz1)
occurs. Below about 27 K a distorted magnetic modulation
with a similar vector kz2 occurs, which is attributed to the
magnetization of the Nd3+ ions by the Mn sublattice. Strong
temperature hysteresis in the occurrence of the
incommensurate magnetic phases in NdMn2O5 was observed
depending on the cooling or heating history of the sample.
Below about 20 K the magnetic structure became of a chiral
type. From spherical neutron polarimetry measurements, the
resulting low-temperature magnetic structure kz3 was
approximated by the general elliptic helix. The parameters
of the magnetic helixlike ellipticity and helical plane
orientation in regard to the crystal structure were
determined. A reorientation of the helix occurs at an
intermediate temperature between 4 and 18 K. A difference
between the population of right- and left-handed chiral
domains of about 0.2 was observed in the as-grown crystal
when cooling without an external electric field. The
magnetic chiral ratio can be changed by the application of
an external electric field of a few kV/cm, revealing strong
magnetoelectric coupling. A linear dependence of the
magnetic chirality on the applied electric field in NdMn2O5
was found. The results are discussed within the frame of the
antisymmetric superexchange model for Dzyaloshinskii-Moriya
interaction.},
cin = {JCNS-FRM-II / MLZ},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6G15 - FRM II / MLZ (POF3-6G15)},
pid = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
experiment = {EXP:(DE-MLZ)POLI-HEIDI-20140101 /
EXP:(DE-MLZ)RESI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000515628700004},
doi = {10.1103/PhysRevB.101.064425},
url = {https://juser.fz-juelich.de/record/888916},
}