TY  - JOUR
AU  - Sun, Yajie
AU  - Wu, Bei
AU  - Wiekenkamp, Inge
AU  - Kooijman, Annemieke M.
AU  - Bol, Roland
TI  - Uranium Vertical and Lateral Distribution in a German Forested Catchment
JO  - Forests
VL  - 11
IS  - 12
SN  - 1999-4907
CY  - Basel
PB  - MDPI
M1  - FZJ-2020-05385
SP  - 1351 -
PY  - 2020
AB  - The natural measurements of uranium (U) are important for establishing natural baseline levels of U in soil. The relations between U and other elements are important to determine the extent of geological origin of soil U. The present study was aimed at providing a three-dimensional view of soil U distribution in a forested catchment (ca. 38.5 ha) in western Germany. The evaluated data, containing 155 sampled points, each with four major soil horizons (L/Of, Oh, A, and B), were collected from two existing datasets. The vertical U distribution, the lateral pattern of U in the catchment, and the occurrence of correlations between U and three groups of elements (nutrient elements, heavy metals, and rare earth elements) were examined. The results showed the median U concentration increased sevenfold from the top horizon L/Of (0.14 mg kg−1) to the B horizon (1.01 mg kg−1), suggesting a geogenic origin of soil U. Overall, soil U concentration was found to be negatively correlated with some plant macronutrients (C, N, K, S, Ca) but positively with others (P, Mg, Cu, Zn, Fe, Mn, Mo). The negative correlations between U and some macronutrients indicated a limited accumulation of plant-derived U in soil, possibly due to low phytoavailability of U. Positive correlations were also found between U concentration and heavy metals (Cr, Co, Ni, Ga, As, Cd, Hg, Pb) or rare earth elements, which further pointed to a geogenic origin of soil U in this forested catchment.
LB  - PUB:(DE-HGF)16
UR  - <Go to ISI:>//WOS:000602172200001
DO  - DOI:10.3390/f11121351
UR  - https://juser.fz-juelich.de/record/889010
ER  -