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@ARTICLE{Liu:889212,
      author       = {Liu, Chang and Shviro, Meital and Gago, Aldo S. and
                      Zaccarine, Sarah F. and Bender, Guido and Gazdzicki, Pawel
                      and Morawietz, Tobias and Biswas, Indro and Rasinski, Marcin
                      and Everwand, Andreas and Schierholz, Roland and
                      Pfeilsticker, Jason and Müller, Martin and Lopes, Pietro P.
                      and Eichel, Rüdiger-A. and Pivovar, Bryan and Pylypenko,
                      Svitlana and Friedrich, K. Andreas and Lehnert, Werner and
                      Carmo, Marcelo},
      title        = {{E}xploring the {I}nterface of {S}kin‐{L}ayered
                      {T}itanium {F}ibers for {E}lectrochemical {W}ater
                      {S}plitting},
      journal      = {Advanced energy materials},
      volume       = {11},
      number       = {8},
      issn         = {1614-6840},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2021-00118},
      pages        = {2002926},
      year         = {2021},
      abstract     = {Water electrolysis is the key to a decarbonized energy
                      system, as it enables the conversion and storage of
                      renewably generated intermittent electricity in the form of
                      hydrogen. However, reliability challenges arising from
                      titanium‐based porous transport layers (PTLs) have
                      hitherto restricted the deployment of next‐generation
                      water‐splitting devices. Here, it is shown for the first
                      time how PTLs can be adapted so that their interface remains
                      well protected and resistant to corrosion across ≈4000 h
                      under real electrolysis conditions. It is also demonstrated
                      that the malfunctioning of unprotected PTLs is a result
                      triggered by additional fatal degradation mechanisms over
                      the anodic catalyst layer beyond the impacts expected from
                      iridium oxide stability. Now, superior durability and
                      efficiency in water electrolyzers can be achieved over
                      extended periods of operation with less‐expensive PTLs
                      with proper protection, which can be explained by the
                      detailed reconstruction of the interface between the
                      different elements, materials, layers, and components
                      presented in this work.},
      cin          = {IEK-14 / IEK-9 / IEK-4},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-14-20191129 / I:(DE-Juel1)IEK-9-20110218 /
                      I:(DE-Juel1)IEK-4-20101013},
      pnm          = {134 - Plasma-Wand-Wechselwirkung (POF4-134) / 123 -
                      Chemische Energieträger (POF4-123)},
      pid          = {G:(DE-HGF)POF4-134 / G:(DE-HGF)POF4-123},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000604739000001},
      doi          = {10.1002/aenm.202002926},
      url          = {https://juser.fz-juelich.de/record/889212},
}