000889747 001__ 889747
000889747 005__ 20230111074316.0
000889747 0247_ $$2doi$$a10.1021/acssuschemeng.0c06019
000889747 0247_ $$2altmetric$$aaltmetric:94674902
000889747 0247_ $$2WOS$$aWOS:000595593500015
000889747 037__ $$aFZJ-2021-00361
000889747 082__ $$a540
000889747 1001_ $$0P:(DE-HGF)0$$aUtomo, Romualdus Nugraha Catur$$b0
000889747 245__ $$aDefined Microbial Mixed Culture for Utilization of Polyurethane Monomers
000889747 260__ $$aWashington, DC$$bACS Publ.$$c2020
000889747 3367_ $$2DRIVER$$aarticle
000889747 3367_ $$2DataCite$$aOutput Types/Journal article
000889747 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1611745321_11439
000889747 3367_ $$2BibTeX$$aARTICLE
000889747 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000889747 3367_ $$00$$2EndNote$$aJournal Article
000889747 500__ $$aKein Post-print verfügbar
000889747 520__ $$aThe end-of-life plastic crisis is very prominent in the research area and even in the public realm. Especially, for plastic polymers that are difficult to recycle via traditional routes such as the polyurethanes (PUs), novel routes should be investigated. In 2015, PU contributed about 16 million metric tons of global plastic waste. While polymer degradation via chemical routes such as solvolysis and pyrolysis are feasible, the challenge of PU chemical recycling is in the varying mixture and composition of its monomers. Here, we propose a biotechnological route to utilize PU hydrolysate as a carbon source for a defined microbial mixed culture. The mixed culture consists of dedicated microbes, each trained to utilize a single PU monomer and further engineered to produce valuable products. While three Pseudomonas putida KT2440 derivatives utilized adipic acid, 1,4-butanediol, and ethylene glycol, respectively, a recently described Pseudomonas sp. TDA1 used 2,4-toluenediamine (TDA) as a sole carbon source. However, TDA clearly inhibited mixed substrate utilization by the mixed culture, and it also has a high intrinsic value. Therefore, TDA reactive extraction before PU monomer utilization was established, allowing full utilization of the remaining PU monomers as carbon sources for rhamnolipid production. The results highlight the potential of (bio)technological plastic upcycling.
000889747 536__ $$0G:(DE-HGF)POF3-581$$a581 - Biotechnology (POF3-581)$$cPOF3-581$$fPOF III$$x0
000889747 588__ $$aDataset connected to CrossRef
000889747 7001_ $$0P:(DE-Juel1)176879$$aLi, Wing-Jin$$b1
000889747 7001_ $$0P:(DE-HGF)0$$aTiso, Till$$b2
000889747 7001_ $$0P:(DE-HGF)0$$aEberlein, Christian$$b3
000889747 7001_ $$0P:(DE-Juel1)180324$$aDoeker, Moritz$$b4
000889747 7001_ $$0P:(DE-HGF)0$$aHeipieper, Hermann J.$$b5
000889747 7001_ $$00000-0001-6551-5695$$aJupke, Andreas$$b6
000889747 7001_ $$0P:(DE-Juel1)176653$$aWierckx, Nick$$b7
000889747 7001_ $$00000-0003-0961-4976$$aBlank, Lars M.$$b8$$eCorresponding author
000889747 773__ $$0PERI:(DE-600)2695697-4$$a10.1021/acssuschemeng.0c06019$$gVol. 8, no. 47, p. 17466 - 17474$$n47$$p17466 - 17474$$tACS sustainable chemistry & engineering$$v8$$x2168-0485$$y2020
000889747 8564_ $$uhttps://juser.fz-juelich.de/record/889747/files/acssuschemeng.0c06019.pdf$$yRestricted
000889747 909CO $$ooai:juser.fz-juelich.de:889747$$pVDB
000889747 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)180324$$aForschungszentrum Jülich$$b4$$kFZJ
000889747 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)176653$$aForschungszentrum Jülich$$b7$$kFZJ
000889747 9130_ $$0G:(DE-HGF)POF3-581$$1G:(DE-HGF)POF3-580$$2G:(DE-HGF)POF3-500$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bKey Technologies$$lKey Technologies for the Bioeconomy$$vBiotechnology$$x0
000889747 9141_ $$y2021
000889747 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bACS SUSTAIN CHEM ENG : 2018$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2020-08-28
000889747 915__ $$0StatID:(DE-HGF)9905$$2StatID$$aIF >= 5$$bACS SUSTAIN CHEM ENG : 2018$$d2020-08-28
000889747 920__ $$lyes
000889747 9201_ $$0I:(DE-Juel1)IBG-1-20101118$$kIBG-1$$lBiotechnologie$$x0
000889747 980__ $$ajournal
000889747 980__ $$aVDB
000889747 980__ $$aI:(DE-Juel1)IBG-1-20101118
000889747 980__ $$aUNRESTRICTED