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@ARTICLE{Utomo:889747,
      author       = {Utomo, Romualdus Nugraha Catur and Li, Wing-Jin and Tiso,
                      Till and Eberlein, Christian and Doeker, Moritz and
                      Heipieper, Hermann J. and Jupke, Andreas and Wierckx, Nick
                      and Blank, Lars M.},
      title        = {{D}efined {M}icrobial {M}ixed {C}ulture for {U}tilization
                      of {P}olyurethane {M}onomers},
      journal      = {ACS sustainable chemistry $\&$ engineering},
      volume       = {8},
      number       = {47},
      issn         = {2168-0485},
      address      = {Washington, DC},
      publisher    = {ACS Publ.},
      reportid     = {FZJ-2021-00361},
      pages        = {17466 - 17474},
      year         = {2020},
      note         = {Kein Post-print verfügbar},
      abstract     = {The end-of-life plastic crisis is very prominent in the
                      research area and even in the public realm. Especially, for
                      plastic polymers that are difficult to recycle via
                      traditional routes such as the polyurethanes (PUs), novel
                      routes should be investigated. In 2015, PU contributed about
                      16 million metric tons of global plastic waste. While
                      polymer degradation via chemical routes such as solvolysis
                      and pyrolysis are feasible, the challenge of PU chemical
                      recycling is in the varying mixture and composition of its
                      monomers. Here, we propose a biotechnological route to
                      utilize PU hydrolysate as a carbon source for a defined
                      microbial mixed culture. The mixed culture consists of
                      dedicated microbes, each trained to utilize a single PU
                      monomer and further engineered to produce valuable products.
                      While three Pseudomonas putida KT2440 derivatives utilized
                      adipic acid, 1,4-butanediol, and ethylene glycol,
                      respectively, a recently described Pseudomonas sp. TDA1 used
                      2,4-toluenediamine (TDA) as a sole carbon source. However,
                      TDA clearly inhibited mixed substrate utilization by the
                      mixed culture, and it also has a high intrinsic value.
                      Therefore, TDA reactive extraction before PU monomer
                      utilization was established, allowing full utilization of
                      the remaining PU monomers as carbon sources for rhamnolipid
                      production. The results highlight the potential of
                      (bio)technological plastic upcycling.},
      cin          = {IBG-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IBG-1-20101118},
      pnm          = {581 - Biotechnology (POF3-581)},
      pid          = {G:(DE-HGF)POF3-581},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000595593500015},
      doi          = {10.1021/acssuschemeng.0c06019},
      url          = {https://juser.fz-juelich.de/record/889747},
}