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@ARTICLE{Tegel:8899,
author = {Tegel, M. and Hummel, F. and Su, Y. and Chatterji, T. and
Brunelli, M. and Johrendt, D.},
title = {{N}on-stoichometry and the magnetic structure of
{S}r2{C}r{O}3{F}e{A}s},
journal = {epl},
volume = {89},
issn = {0302-072X},
address = {Les Ulis},
publisher = {EDP Sciences},
reportid = {PreJuSER-8899},
pages = {37006},
year = {2010},
note = {This work was financially supported by the German Research
Foundation (DFG). MT would like to thank Dr K. ROMER for
financial support.},
abstract = {The iron arsenide Sr2CrO3FeAs with the tetragonal
Sr2GaO3CuS-type structure was synthesized and its crystal
structure re-determined by neutron powder diffraction. In
contrast to previous X-ray crystallographic studies, a mixed
occupancy of chromium and iron was found within the FeAs4/4
layer (93 +/- $1\%Fe$ : 7 +/- $1\%Cr).$ We suggest that the
partial Cr-doping at the Fe site is the reason for the
absence of a spin-density-wave anomaly and superconductivity
in this compound. Additional experiments via neutron
polarization analysis revealed short-range spin correlations
below similar to 100 K and long-range antiferromagnetic
ordering below T-N = 36 K with a magnetic propagation vector
of q = (1/2, 1/2, 0). The Cr3+ -ions form a collinear
magnetic structure of the C-type in the magnetic space group
C(P)mma' (a' = a-b, b' = a+b, c' = c), where Cr3+-ions
occupy the 4g (0, 1/4, z) Wyckoff position. The magnetic
moments are aligned along the orthorhombic a'-axis. At 3.5
K, an ordered magnetic moment of 2.75 +/- 0.05 mu B for the
Cr3+ -sublattice was refined.},
keywords = {J (WoSType)},
cin = {IFF-4 / IFF-5 / Jülich Centre for Neutron Science JCNS
(JCNS) ; JCNS},
ddc = {530},
cid = {I:(DE-Juel1)VDB784 / I:(DE-Juel1)VDB785 /
I:(DE-Juel1)JCNS-20121112},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung / Großgeräte für die Forschung
mit Photonen, Neutronen und Ionen (PNI)},
pid = {G:(DE-Juel1)FUEK505 / G:(DE-Juel1)FUEK415},
experiment = {EXP:(DE-MLZ)DNS-20140101},
shelfmark = {Physics, Multidisciplinary},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000274848600020},
doi = {10.1209/0295-5075/89/37006},
url = {https://juser.fz-juelich.de/record/8899},
}