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@ARTICLE{Schilling:889917,
author = {Schilling, Johannes and Horend, Christian and Bardow,
André},
title = {{I}ntegrating superstructure‐based design of molecules,
processes, and flowsheets},
journal = {AIChE journal},
volume = {66},
number = {5},
issn = {1547-5905},
address = {Hoboken, NJ},
publisher = {Wiley},
reportid = {FZJ-2021-00525},
pages = {e16903},
year = {2020},
abstract = {The key to many chemical and energy conversion processes is
the choice of the right molecule, for example, used as
working fluid. However, the choice of the molecule is
inherently coupled to the choice of the right process
flowsheet. In this work, we integrate superstructure‐based
flowsheet design into the design of processes and molecules.
The thermodynamic properties of the molecule are modeled by
the PC‐SAFT equation of state. Computer‐aided molecular
design enables considering the molecular structure as degree
of freedom in the process optimization. To consider the
process flowsheet as additional degree of freedom, a
superstructure of the process is used. The method results in
the optimal molecule, process, and flowsheet. We demonstrate
the method for the design of an organic Rankine cycle
considering flowsheet options for regeneration, reheating,
and turbine bleeding. The presented method provides a
user‐friendly tool to solve the integrated design problem
of processes, molecules, and process flowsheets.},
cin = {IEK-10},
ddc = {660},
cid = {I:(DE-Juel1)IEK-10-20170217},
pnm = {899 - ohne Topic (POF3-899)},
pid = {G:(DE-HGF)POF3-899},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000507411400001},
doi = {10.1002/aic.16903},
url = {https://juser.fz-juelich.de/record/889917},
}