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@ARTICLE{Habash:889944,
author = {Habash, Samer S. and Brass, Hannah and Klein, Andreas and
Klebl, David P. and Weber, Tim Moritz and Classen, Thomas
and Pietruszka, Jörg and Grundler, Florian M. W. and
Schleker, A. Sylvia S.},
title = {{N}ovel {P}rodiginine {D}erivatives {D}emonstrate
{B}ioactivities on {P}lants, {N}ematodes, and {F}ungi},
journal = {Frontiers in Functional Plant Ecology},
volume = {11},
issn = {1664-462X},
address = {Lausanne},
publisher = {Frontiers Media88991},
reportid = {FZJ-2021-00550},
pages = {579807},
year = {2020},
abstract = {Bacterial metabolites represent an invaluable source of
bioactive molecules which can be used as such or serve as
chemical frameworks for developing new antimicrobial
compounds for various applications including crop protection
against pathogens. Prodiginines are tripyrrolic, red-colored
compounds produced by many bacterial species. Recently, due
to the use of chemical-, bio-, or mutasynthesis, a novel
group of prodiginines was generated. In our study, we
perform different assays to evaluate the effects of
prodigiosin and five derivatives on nematodes and plant
pathogenic fungi as well as on plant development. Our
results showed that prodigiosin and the derivatives were
active against the bacterial feeding nematode Caenorhabditis
elegans in a concentration- and derivative-dependent manner
while a direct effect on infective juveniles of the plant
parasitic nematode Heterodera schachtii was observed for
prodigiosin only. All compounds were found to be active
against the plant pathogenic fungi Phoma lingam and
Sclerotinia sclerotiorum. Efficacy varied depending on
compound concentration and chemical structure. We observed
that prodigiosin (1), the 12 ring- 9, and hexenol 10
derivatives are neutral or even positive for growth of
Arabidopsis thaliana depending on the applied compound
concentration, whereas other derivatives appear to be
suppressive. Our infection assays revealed that the total
number of developed H. schachtii individuals on A. thaliana
was decreased to $50\%$ in the presence of compounds 1 or 9.
Furthermore, female nematodes and their associated syncytia
were smaller in size. Prodiginines seem to indirectly
inhibit H. schachtii parasitism of the plant. Further
research is needed to elucidate their mode of action. Our
results indicate that prodiginines are promising metabolites
that have the potential to be developed into novel
antinematodal and antifungal agents.},
cin = {IBOC / IBG-1},
ddc = {570},
cid = {I:(DE-Juel1)IBOC-20090406 / I:(DE-Juel1)IBG-1-20101118},
pnm = {583 - Innovative Synergisms (POF3-583)},
pid = {G:(DE-HGF)POF3-583},
typ = {PUB:(DE-HGF)16},
pubmed = {33178246},
UT = {WOS:000584806100001},
doi = {10.3389/fpls.2020.579807},
url = {https://juser.fz-juelich.de/record/889944},
}