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@ARTICLE{Riedel:889968,
author = {Riedel, M. and Heddrich, M. P. and Ansar, A. and Fang, Q.
and Blum, Ludger and Friedrich, K. A.},
title = {{P}ressurized operation of solid oxide electrolysis stacks:
{A}n experimental comparison of the performance of 10-layer
stacks with fuel electrode and electrolyte supported cell
concepts},
journal = {Journal of power sources},
volume = {475},
issn = {0378-7753},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2021-00571},
pages = {228682 -},
year = {2020},
abstract = {The electrochemical behavior of two different types of
planar 10-layer solid oxide cell (SOC) stacks with having
either fuel electrode supported cells or electrolyte
supported cells, are examined under steam, co- and CO2
electrolysis at elevated pressures of up to 8 bar.
Experiments with steady-state and dynamically recorded
U(i)-characteristics are performed in order to evaluate the
performances over a wide temperature range and for different
operating conditions. Furthermore, the influence of the
operating pressure is quantified via the temperature and
pressure dependency of the related ASR values of each stack.
Impedance analysis is conducted in order to investigate the
major differences and the pressure effect on the specific
process resistances during steam and CO2 electrolysis.In
case of the stack with fuel electrode supported cells, the
ASR is found to decrease significantly at elevated pressure
leading to an overall performance gain, whereas the stack
with electrolyte supported cells shows a minor pressure
effect. An impedance study shows that the diffusion and
activation resistances are significantly affected when
conducting CO2 instead of H2O electrolysis for both stack
concepts. Furthermore, the pressure sensitivity is found to
be more dominant during CO2 electrolysis than during pure
steam electrolysis operation.},
cin = {IEK-14},
ddc = {620},
cid = {I:(DE-Juel1)IEK-14-20191129},
pnm = {135 - Fuel Cells (POF3-135)},
pid = {G:(DE-HGF)POF3-135},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000573641500001},
doi = {10.1016/j.jpowsour.2020.228682},
url = {https://juser.fz-juelich.de/record/889968},
}