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@ARTICLE{Lin:890046,
author = {Lin, Rui and Tang, Shenghao and Diao, Xiaoyu and Zhong, Di
and Chen, Liang and Froning, Dieter and Hao, Zhixian},
title = {{D}etailed optimization of multiwall carbon nanotubes doped
microporous layer in polymer electrolyte membrane fuel cells
for enhanced performance},
journal = {Applied energy},
volume = {274},
issn = {0306-2619},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2021-00640},
pages = {115214 -},
year = {2020},
abstract = {Polymer electrolyte membrane fuel cell is a promising
renewable energy technology. In order to further enhance the
output performance improvement caused by the doping of
multiwall carbon nanotubes in microporous layers, in this
study, detailed optimization of microporous layers
containing multiwall carbon nanotubes is accomplished. The
synergy effects of carbon powder types, contents and
diameters of multiwall carbon nanotubes, and microporous
layer loadings are considered for the first time. The
optimal composition under different humidity is obtained. It
is found that among the four factors, carbon powder types
have the greatest impact on the performance. The fuel cells
containing thick multiwall carbon nanotubes exhibit more
stable performance with the change of humidity. Microporous
layers with large content of multiwall carbon nanotubes (15
$wt\%)$ promise better performance. The performance of
microporous layer with the carbon powder of XC-72 is the
worst due to inferior mass transfer and increased ohm
resistance. The fuel cell with the optimized microporous
layer exhibits excellent performance, under the temperature
of 80 °C and 0.8 bar back pressure, the current density at
0.6 V is up to 1900 mA/cm2, and the max power density
reaches 1180 mW/cm2. The significant improvement of
performance can be attributed to favorable porous structure
along with enhanced mass transfer and improved
conductivity.},
cin = {IEK-14},
ddc = {620},
cid = {I:(DE-Juel1)IEK-14-20191129},
pnm = {135 - Fuel Cells (POF3-135)},
pid = {G:(DE-HGF)POF3-135},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000545317600002},
doi = {10.1016/j.apenergy.2020.115214},
url = {https://juser.fz-juelich.de/record/890046},
}