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@ARTICLE{Zeng:890183,
      author       = {Zeng, Linxiang and Chen, Shi and Forberich, Karen and
                      Brabec, Christoph J. and Mai, Yaohua and Guo, Fei},
      title        = {{C}ontrolling the crystallization dynamics of photovoltaic
                      perovskite layers on larger-area coatings},
      journal      = {Energy $\&$ environmental science},
      volume       = {13},
      number       = {12},
      issn         = {1754-5706},
      address      = {Cambridge},
      publisher    = {RSC Publ.},
      reportid     = {FZJ-2021-00772},
      pages        = {4666 - 4690},
      year         = {2020},
      abstract     = {As perovskite solar cells are highly efficient and already
                      meet the efficiency requirement for renewable
                      powergeneration, more attention is given to technological
                      barriers such as scalability and stability. In particular,
                      thelarge efficiency losses associated with upscaling
                      lab-scale devices to large-area modules represents one ofthe
                      major hurdles for commercialization. Given the essential
                      role of the perovskite films in the deviceperformance, it is
                      of critical importance to develop reliable crystallization
                      protocols to deposit high-qualityperovskite layers via
                      scalable methods. This review summarizes recent advances in
                      emerging crystallizationprotocols for the large-scale
                      deposition of perovskite thin films. The unique merits of
                      the well-developedcrystallization strategies, including
                      antisolvent, gas quenching, vacuum quenching, etc., are
                      carefully analyzedand discussed. We highlight that,
                      independent of the coating method, creating intermediate
                      phases todecouple the otherwise overlapped solution coating
                      and crystal growth is essential to realize
                      homogeneouscoatings of perovskite thin films. Strategies for
                      enhancing the crystal morphology of perovskite films
                      arepresented as well, which is vitally important to realize
                      reproducible manufacturing of large-area modules.
                      Thistutorial review assists the screening and development of
                      robust crystallization strategies for scalabledeposition of
                      high-quality perovskite films for photovoltaic
                      applications.},
      cin          = {IEK-11},
      ddc          = {690},
      cid          = {I:(DE-Juel1)IEK-11-20140314},
      pnm          = {121 - Solar cells of the next generation (POF3-121)},
      pid          = {G:(DE-HGF)POF3-121},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000599751100009},
      doi          = {10.1039/D0EE02575E},
      url          = {https://juser.fz-juelich.de/record/890183},
}