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@ARTICLE{Zanatta:890231,
author = {Zanatta, Marco and Bozem, Heiko and Köllner, Franziska and
Schneider, Johannes and Kunkel, Daniel and Hoor, Peter and
de Faria, Julia and Petzold, Andreas and Bundke, Ulrich and
Hayden, Katherine and Staebler, Ralf M. and Schulz, Hannes
and Herber, Andreas B.},
title = {{A}irborne survey of trace gases and aerosols over the
{S}outhern {B}altic {S}ea: from clean marine boundary layer
to shipping corridor effect},
journal = {Tellus / B},
volume = {72},
number = {1},
issn = {1600-0889},
address = {Abingdon},
publisher = {Taylor $\&$ Francis},
reportid = {FZJ-2021-00818},
pages = {1 - 24},
year = {2020},
abstract = {The influence of shipping on air quality over the Southern
Baltic Sea was investigated by characterizing the horizontal
and vertical distribution of aerosols and trace gases using
airborne measurements in the summer of 2015. Generally,
continental and anthropogenic emissions affected the
vertical distribution of atmospheric pollutants, leading to
pronounced stratification in and above the marine boundary
layer and controlling the aerosol extinction. Marine traffic
along the shipping corridor “Kadet Fairway” in the
Arkona Basin is shown to influence the presence and
properties of both trace gases and aerosol particles in the
lowest atmospheric layer. Total particle number
concentration and NOy mixing ratio increased in the corridor
plumes, relative to background, by a factor 1.55 and 3.45,
respectively. Titration, triggered by the enhanced presence
of nitrogen compounds, led to a median ozone depletion of
$19\%$ in the corridor plumes. The enforcement of the
Sulphur Emission Control Area (SECA) might be responsible
for the minor sulphur dioxide increase $(20\%)$ in the
corridor plumes. Ship traffic caused a minor enhancement of
black carbon mass concentration, estimated to be around
$10\%.$ The study of individual ship plumes indicated that
ship emitted aerosol was substantially different from
background aerosol: fresh ship exhaust was preferentially
enriched in aerosol particles with diameters below 100 nm
and in black carbon particles with core diameters above
300-400 nm. With the present work the impact of marine
traffic on the concentration and properties of atmospheric
components within the marine boundary layer over the open
water of the Southern Baltic Sea is assessed with airborne
observations for the first time. Due to the high uncertainty
affecting the estimations of ship emissions, this dataset
represents a valuable reference for the assessment of ship
emission inventories and related environmental-climatic
impacts on the Southern Baltic Sea},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {243 - Tropospheric trace substances and their
transformation processes (POF3-243)},
pid = {G:(DE-HGF)POF3-243},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000600212000001},
doi = {10.1080/16000889.2019.1695349},
url = {https://juser.fz-juelich.de/record/890231},
}