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@ARTICLE{Papagiannopoulos:890358,
      author       = {Papagiannopoulos, Aristeidis and Vlassi, Eleni and Pispas,
                      Stergios and Tsitsilianis, Constantinos and Radulescu,
                      Aurel},
      title        = {{P}olyethylene {O}xide {H}ydrogels {C}rosslinked by
                      {P}eroxide for the {C}ontrolled {R}elease of {P}roteins},
      journal      = {Macromol},
      volume       = {1},
      number       = {1},
      issn         = {2673-6209},
      address      = {Basel},
      publisher    = {MDPI AG},
      reportid     = {FZJ-2021-00903},
      pages        = {37-48},
      year         = {2021},
      abstract     = {Crosslinking of polyethylene oxide (PEO) using a peroxide
                      in the melt is employed to synthesize soft hydrogels with
                      the ability of controlled release of proteins. The
                      viscoelastic properties of the swollen networks confirm the
                      elastic nature of the synthesized material and they are in
                      agreement with swelling characteristics. The hydrogels have
                      mesh sizes at the nm scale as it is estimated by swelling
                      measurements and measured by small angle neutron scattering
                      (SANS). Diffusion of bovine serum albumin (BSA) and lysozyme
                      (LYZ) out of the hydrogels is restricted by the presence of
                      the network. The diffusion coefficient in the hydrogels is
                      lower for BSA in comparison to LYZ, while in both cases it
                      drops as the mesh size of the network becomes smaller. This
                      study introduces the use of peroxide-crosslinked PEO
                      networks in the investigation of protein transport within
                      hydrogels, the development of hydrogel-based protein
                      delivery patches and polymeric constructs},
      cin          = {JCNS-FRM-II / MLZ / JCNS-1},
      ddc          = {570},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3 /
                      I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
                      (POF4-6G4)},
      pid          = {G:(DE-HGF)POF4-6G4},
      experiment   = {EXP:(DE-MLZ)KWS2-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001204340100001},
      doi          = {10.3390/macromol1010004},
      url          = {https://juser.fz-juelich.de/record/890358},
}