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@ARTICLE{Borzutzki:890455,
      author       = {Borzutzki, Kristina Kerstin and Winter, Martin and
                      Brunklaus, Gunther},
      title        = {{I}mproving the {NMC}111∣ {P}olymer {E}lectrolyte
                      {I}nterface by {C}athode {C}omposition and {P}rocessing},
      journal      = {Journal of the Electrochemical Society},
      volume       = {167},
      number       = {7},
      issn         = {0013-4651},
      address      = {Bristol},
      publisher    = {IOP Publishing},
      reportid     = {FZJ-2021-00971},
      pages        = {070546},
      year         = {2020},
      abstract     = {Despite significant improvements of polymer electrolyte
                      properties, the interfaces towards the electrodes often
                      yield high interfacial resistances due to poor contacts,
                      which are bottlenecks for application of newly developed
                      polymer, ceramic or composite electrolytes in lithium metal
                      batteries (LMBs). Herein, the impact of processing as well
                      as slurry composition of LiNi1/3Co1/3Mn1/3O2 (NMC111) based
                      composite cathodes on the achievable electrochemical C-rate
                      performance of LMBs based on quasi-solid single ion
                      conducting polymer electrolytes (SIPE) is demonstrated.
                      Composite cathodes with varying types and amounts of
                      lithiated species are fabricated and systematically
                      compared. Among all considered electrodes, cathodes with an
                      addition of 5 $wt\%$ lithiated terephthalic acid (TA Li)
                      yield the highest discharge capacity of 91 mAhg−1 at 1 C
                      for Li metalmidSIPEmidNMC111 cells. Furthermore, similar
                      cells operated with cathodes whose pores are impregnated
                      with 5 $wt\%$ SIPE via drop/spin coating even provide a
                      specific discharge capacity of 113 mAhg−1 at 1 C, thereby
                      clearly highlighting the benefit of the selected processing
                      strategy to realize cathodes with substantially improved
                      charge carrier transport networks.},
      cin          = {IEK-12},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000522880100002},
      doi          = {10.1149/1945-7111/ab7fb5},
      url          = {https://juser.fz-juelich.de/record/890455},
}