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@ARTICLE{Sun:891312,
author = {Sun, Shijing and Tiihonen, Armi and Oviedo, Felipe and Liu,
Zhe and Thapa, Janak and Zhao, Yicheng and Hartono, Noor
Titan P. and Goyal, Anuj and Heumueller, Thomas and Batali,
Clio and Encinas, Alex and Yoo, Jason J. and Li, Ruipeng and
Ren, Zekun and Peters, I. Marius and Brabec, Christoph J.
and Bawendi, Moungi G. and Stevanovic, Vladan and Fisher,
John and Buonassisi, Tonio},
title = {{A} data fusion approach to optimize compositional
stability of halide perovskites},
journal = {Matter},
volume = {4},
number = {4},
issn = {2590-2385},
address = {[New York, NY]},
publisher = {Elsevier},
reportid = {FZJ-2021-01419},
pages = {1305-1322},
year = {2021},
abstract = {Despite recent intensive efforts to improve the
environmental stability of halide perovskite materials for
energy harvesting and conversion, traditional
trial-and-error explorations face bottlenecks in the
navigation of vast chemical and compositional spaces. We
develop a closed-loop optimization framework that seamlessly
marries data from first-principle calculations and
high-throughput experimentation into a single machine
learning algorithm. This framework enables us to achieve
rapid optimization of compositional stability for
CsxMAyFA1−x−yPbI3 perovskites while taking the human out
of the decision-making loop. We envision that this data
fusion approach is generalizable to directly tackle
challenges in designing multinary materials, and we hope
that our successful showcase on perovskites will encourage
researchers in other fields to incorporate knowledge of
physics into the search algorithms, applying hybrid machine
learning models to guide discovery of materials in
high-dimensional spaces.},
cin = {IEK-11},
ddc = {600},
cid = {I:(DE-Juel1)IEK-11-20140314},
pnm = {121 - Photovoltaik und Windenergie (POF4-121)},
pid = {G:(DE-HGF)POF4-121},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000637800400003},
doi = {10.1016/j.matt.2021.01.008},
url = {https://juser.fz-juelich.de/record/891312},
}