000008915 001__ 8915 000008915 005__ 20230426083016.0 000008915 0247_ $$2DOI$$a10.1103/PhysRevB.81.054434 000008915 0247_ $$2WOS$$aWOS:000274998000084 000008915 0247_ $$2Handle$$a2128/10999 000008915 037__ $$aPreJuSER-8915 000008915 041__ $$aeng 000008915 082__ $$a530 000008915 084__ $$2WoS$$aPhysics, Condensed Matter 000008915 1001_ $$0P:(DE-Juel1)VDB63896$$aSasioglu, E.$$b0$$uFZJ 000008915 245__ $$aWannier-function approach to spin excitations in solids 000008915 260__ $$aCollege Park, Md.$$bAPS$$c2010 000008915 300__ $$a054434 000008915 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article 000008915 3367_ $$2DataCite$$aOutput Types/Journal article 000008915 3367_ $$00$$2EndNote$$aJournal Article 000008915 3367_ $$2BibTeX$$aARTICLE 000008915 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000008915 3367_ $$2DRIVER$$aarticle 000008915 440_0 $$04919$$aPhysical Review B$$v81$$x1098-0121$$y5 000008915 500__ $$aFruitful discussions with Y. Mokrousov, G. Bihlmayer, M. Niesert, A. Gierlich, T. Miyake, and F. Aryasetiawan are gratefully acknowledged. This work was funded in part by the EU through the Nanoquanta Network of Excellence (Grant No. NMP4-CT-2004-500198), the European Theoretical Spectroscopy Facility e-I3 (Grant No. INFRA-2007-211956), and by the Deutsche Forschungsgemeinschaft through the Priority Programme 1145. 000008915 520__ $$aWe present a computational scheme to study spin excitations in magnetic materials from first principles. The central quantity is the transverse spin susceptibility, from which the complete excitation spectrum, including single-particle spin-flip Stoner excitations and collective spin-wave modes, can be obtained. The susceptibility is derived from many-body perturbation theory and includes dynamic correlation through a summation over ladder diagrams that describe the coupling of electrons and holes with opposite spins. In contrast to earlier studies, we do not use a model potential with adjustable parameters for the electron-hole interaction but employ the random-phase approximation. To reduce the numerical cost for the calculation of the four-point scattering matrix we perform a projection onto maximally localized Wannier functions, which allows us to truncate the matrix efficiently by exploiting the short spatial range of electronic correlation in the partially filled d or f orbitals. Our implementation is based on the full-potential linearized augmented-plane-wave method. Starting from a ground-state calculation within the local-spin-density approximation (LSDA), we first analyze the matrix elements of the screened Coulomb potential in the Wannier basis for the 3d transition-metal series. In particular, we discuss the differences between a constrained nonmagnetic and a proper spin-polarized treatment for the ferromagnets Fe, Co, and Ni. The spectrum of single-particle and collective spin excitations in fcc Ni is then studied in detail. The calculated spin-wave dispersion is in good overall agreement with experimental data and contains both an acoustic and an optical branch for intermediate wave vectors along the [1 0 0] direction. In addition, we find evidence for a similar double-peak structure in the spectral function along the [1 1 1] direction. To investigate the influence of static correlation we finally consider LSDA+U as an alternative starting point and show that, together with an improved description of the Fermi surface, it yields a more accurate quantitative value for the spin-wave stiffness constant, which is overestimated in the LSDA. 000008915 536__ $$0G:(DE-Juel1)FUEK412$$2G:(DE-HGF)$$aGrundlagen für zukünftige Informationstechnologien$$cP42$$x0 000008915 536__ $$0G:(EU-Grant)211956$$aETSF - European Theoretical Spectroscopy Facility I3 (211956)$$c211956$$fFP7-INFRASTRUCTURES-2007-1$$x1 000008915 542__ $$2Crossref$$i2010-02-22$$uhttp://link.aps.org/licenses/aps-default-license 000008915 588__ $$aDataset connected to Web of Science 000008915 650_7 $$2WoSType$$aJ 000008915 7001_ $$0P:(DE-HGF)0$$aSchindlmayr, A.$$b1 000008915 7001_ $$0P:(DE-Juel1)VDB418$$aFriedrich, C.$$b2$$uFZJ 000008915 7001_ $$0P:(DE-Juel1)130643$$aFreimuth, F.$$b3$$uFZJ 000008915 7001_ $$0P:(DE-Juel1)130548$$aBlügel, S.$$b4$$uFZJ 000008915 77318 $$2Crossref$$3journal-article$$a10.1103/physrevb.81.054434$$bAmerican Physical Society (APS)$$d2010-02-22$$n5$$p054434$$tPhysical Review B$$v81$$x1098-0121$$y2010 000008915 773__ $$0PERI:(DE-600)2844160-6$$a10.1103/PhysRevB.81.054434$$gVol. 81, p. 054434$$n5$$p054434$$q81<054434$$tPhysical review / B$$v81$$x1098-0121$$y2010 000008915 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevB.81.054434 000008915 8564_ $$uhttps://juser.fz-juelich.de/record/8915/files/PhysRevB.81.054434.pdf$$yOpenAccess 000008915 8564_ $$uhttps://juser.fz-juelich.de/record/8915/files/PhysRevB.81.054434.gif?subformat=icon$$xicon$$yOpenAccess 000008915 8564_ $$uhttps://juser.fz-juelich.de/record/8915/files/PhysRevB.81.054434.jpg?subformat=icon-180$$xicon-180$$yOpenAccess 000008915 8564_ $$uhttps://juser.fz-juelich.de/record/8915/files/PhysRevB.81.054434.jpg?subformat=icon-700$$xicon-700$$yOpenAccess 000008915 8564_ $$uhttps://juser.fz-juelich.de/record/8915/files/PhysRevB.81.054434.pdf?subformat=pdfa$$xpdfa$$yOpenAccess 000008915 909CO $$ooai:juser.fz-juelich.de:8915$$pdnbdelivery$$pec_fundedresources$$pVDB$$pdriver$$popen_access$$popenaire 000008915 9141_ $$y2010 000008915 915__ $$0LIC:(DE-HGF)APS-112012$$2HGFVOC$$aAmerican Physical Society Transfer of Copyright Agreement 000008915 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess 000008915 915__ $$0StatID:(DE-HGF)0010$$aJCR/ISI refereed 000008915 9131_ $$0G:(DE-Juel1)FUEK412$$aDE-HGF$$bSchlüsseltechnologien$$kP42$$lGrundlagen für zukünftige Informationstechnologien (FIT)$$vGrundlagen für zukünftige Informationstechnologien$$x0 000008915 9201_ $$0I:(DE-Juel1)VDB781$$d31.12.2010$$gIFF$$kIFF-1$$lQuanten-Theorie der Materialien$$x0 000008915 9201_ $$0I:(DE-Juel1)IAS-1-20090406$$gIAS$$kIAS-1$$lQuanten-Theorie der Materialien$$x1$$zIFF-1 000008915 9201_ $$0I:(DE-82)080009_20140620$$gJARA$$kJARA-FIT$$lJülich-Aachen Research Alliance - Fundamentals of Future Information Technology$$x2 000008915 9201_ $$0I:(DE-Juel1)VDB1346$$gJARA$$kJARA-HPC$$lJülich Aachen Research Alliance - High-Performance Computing$$x3 000008915 970__ $$aVDB:(DE-Juel1)118206 000008915 9801_ $$aFullTexts 000008915 980__ $$aVDB 000008915 980__ $$aConvertedRecord 000008915 980__ $$ajournal 000008915 980__ $$aI:(DE-Juel1)PGI-1-20110106 000008915 980__ $$aI:(DE-Juel1)IAS-1-20090406 000008915 980__ $$aI:(DE-82)080009_20140620 000008915 980__ $$aI:(DE-82)080012_20140620 000008915 980__ $$aUNRESTRICTED 000008915 981__ $$aI:(DE-Juel1)PGI-1-20110106 000008915 981__ $$aI:(DE-Juel1)IAS-1-20090406 000008915 981__ $$aI:(DE-Juel1)VDB881 000008915 981__ $$aI:(DE-Juel1)VDB1346 000008915 999C5 $$1T. 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Pines$$2Crossref$$oD. Pines The Many Body Problem 1962$$tThe Many Body Problem$$y1962 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1080/00018737000101201 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.43.2029 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.54.227 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.62.1157 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevB.61.R858 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.82.2579 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.91.147201 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.99.087202 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1103/PhysRevLett.102.177206 000008915 999C5 $$2Crossref$$9-- missing cx lookup --$$a10.1088/0953-8984/16/41/023