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@ARTICLE{Kowalski:891533,
author = {Kowalski, Piotr and He, Zhengda and Cheong, Oskar},
title = {{E}lectrode and {E}lectrolyte {M}aterials {F}rom
{A}tomistic {S}imulations: {P}roperties of {L}ix{FEPO}4
{E}lectrode and {Z}ircon-{B}ased {I}onic {C}onductors},
journal = {Frontiers in energy research},
volume = {9},
issn = {2296-598X},
address = {Lausanne},
publisher = {Frontiers Media},
reportid = {FZJ-2021-01586},
pages = {653542},
year = {2021},
abstract = {LixFePO4 orthophosphates and fluorite- and pyrochlore-type
zirconate materials are widely considered as functional
compounds in energy storage devices, either as electrode or
solid state electrolyte. These ceramic materials show
enhanced cation exchange and anion conductivity properties
that makes them attractive for various energy applications.
In this contribution we discuss thermodynamic properties of
LixFePO4 and yttria-stabilized zirconia compounds, including
formation enthalpies, stability, and solubility limits. We
found that at ambient conditions LixFePO4 has a large
miscibility gap, which is consistent with existing
experimental evidence. We show that cubic zirconia becomes
stabilized with Y content of $~8\%,$ which is in line with
experimental observations. The computed activation energy of
0.92eV and ionic conductivity for oxygen diffusion in
yttria-stabilized zirconia are also in line with the
measured data, which shows that atomistic modeling can be
applied for accurate prediction of key materials properties.
We discuss these results with the existing simulation-based
data on these materials produced by our group over the last
decade. Last, but not least, we discuss similarities of the
considered compounds in considering them as materials for
energy storage and radiation damage resistant matrices for
immobilization of radionuclides.},
cin = {IEK-13 / JARA-ENERGY / JARA-HPC},
ddc = {333.7},
cid = {I:(DE-Juel1)IEK-13-20190226 / $I:(DE-82)080011_20140620$ /
I:(DE-Juel1)VDB1346},
pnm = {122 - Elektrochemische Energiespeicherung (POF4-122)},
pid = {G:(DE-HGF)POF4-122},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000639424900001},
doi = {10.3389/fenrg.2021.653542},
url = {https://juser.fz-juelich.de/record/891533},
}