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@ARTICLE{Popov:891726,
author = {Popov, A. G. and Golovnia, O. A. and Gaviko, V. S. and
Vasilenko, D. Yu and Bratushev, D. Yu and Balaji, V. I.
Nithin and Kovacs, Andras and Pradeep, K. G. and Gopalan,
R.},
title = {{D}evelopment of high-coercivity state in high-energy and
high-temperature {S}m-{C}o-{F}e-{C}u-{Z}r magnets upon step
cooling},
journal = {Journal of alloys and compounds},
volume = {820},
issn = {0925-8388},
address = {Lausanne},
publisher = {Elsevier},
reportid = {FZJ-2021-01699},
pages = {153103 -},
year = {2020},
abstract = {The work compares the peculiarities of the high-coercivity
state formation in the Sm-Co-Fe-Cu-Zr high-temperature and
high-energy permanent magnets (HTPM and HEPM) in the course
of the heat treatment with the stepwise decreasing
temperature from 830 to 400 °C. Two types of magnets with
varying Fe concentration, i.e., Sm(Co0.88-xFexCu0.09Zr0.03)7
with x = 0–0.12 (the HTPMs) and Sm(Co0.91-xFexCu0.06
Zr0.03)7.5 with x = 0.24–0.33 (the HEPMs) were studied at
different temperatures of heat treatment for phase formation
by x-ray diffraction followed by magnetic property
measurements. Microstructure characterization was performed
using transmission electron microscopy, whereas the
three-dimensional elemental distribution at near-atomic
scale was obtained using atom probe tomography. In HEPMs,
the main increase in coercivity and relaxation of stresses
accompanied by intensive enrichment of the 1:5 phase in Cu
are observed at high temperatures (Т ≈ 700 °C). In
HTPMs, the coercivity monotonously increases in the entire
temperature range of the slow cooling from 700 to 400 °C at
a rate of 0.5 °C/s. At the temperature close to the Curie
temperature (∼550 °C) of the Sm(Co,Cu)5-type phase, the
anomaly of the coercivity increment has been observed. The
interphase stresses grow and the elemental redistribution
appears to be accelerated simultaneously. The non-uniform Cu
distribution in the 1:5 phase can be described by the
formation of Cu-rich interlayers at the interface of the
Sm(Co,Cu)5 and Sm2(Co,Fe)17-type phases.},
cin = {ER-C-1},
ddc = {540},
cid = {I:(DE-Juel1)ER-C-1-20170209},
pnm = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000507854700026},
doi = {10.1016/j.jallcom.2019.153103},
url = {https://juser.fz-juelich.de/record/891726},
}