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@ARTICLE{Yoshino:891836,
      author       = {Yoshino, K. and Suzuki, K. and Yamada, Y. and Satoh, T. and
                      Finsterbusch, M. and Fujita, K. and Kamiya, T. and Yamazaki,
                      A. and Mima, K. and Hirayama, M. and Kanno, R.},
      title        = {{L}ithium distribution analysis in all-solid-state lithium
                      battery using microbeam particle-induced {X}-ray emission
                      and particle-induced gamma-ray emission techniques},
      journal      = {International journal of PIXE},
      volume       = {27},
      number       = {01n02},
      issn         = {1793-6616},
      address      = {Singapore},
      publisher    = {World Scientific},
      reportid     = {FZJ-2021-01759},
      pages        = {11 - 20},
      year         = {2017},
      abstract     = {For confirming the feasibility of micrometer scale analysis
                      of lithium distribution in the all-solid-state lithium
                      battery using a sulfide-based solid electrolyte, the
                      cross-section of pellet type battery was analyzed by
                      microbeam particle-induced X-ray emission (PIXE) and
                      particle-induced gamma-ray emission (PIGE) measurements. A
                      three-layered pellet-type battery (cathode: LiNbO3-coated
                      LiCoO2+Li10GeP2S12/solid electrolyte: Li10GeP2S12/anode:
                      TiS2+Li10GeP2S12) was prepared for the measurements. Via
                      elemental mapping of the cross-section of the prepared
                      battery, the difference in the yields of gamma rays from the
                      7Li(p,p′γ)7Li inelastic scattering (i.e., the lithium
                      concentrations) between the composite electrodes and the
                      solid electrolyte layer was clarified. The difference in the
                      number of lithium ions at the composite anode/solid
                      electrolyte interface of (Δn=0.26×10−4 mol) in the
                      battery can be clearly detected by the microbeam PIGE
                      technique. Therefore, lithium distribution analysis with a
                      micrometer-scale spatial resolution is demonstrated. Further
                      analysis of the cathode/anode composite electrodes with the
                      different states of charge could provide important
                      information to design a composite for high-performance
                      all-solid-state lithium batteries.},
      cin          = {IEK-1},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.1142/S012908351850002X},
      url          = {https://juser.fz-juelich.de/record/891836},
}