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@ARTICLE{Rosati:891840,
      author       = {Rosati, Bernadette and Paul, Andreas and Iversen, Emil Mark
                      and Massling, Andreas and Bilde, Merete},
      title        = {{R}econciling atmospheric water uptake by hydrate forming
                      salts},
      journal      = {Environmental science},
      volume       = {22},
      number       = {8},
      issn         = {2050-7895},
      address      = {Cambridge},
      publisher    = {RSC Publ.},
      reportid     = {FZJ-2021-01763},
      pages        = {1759 - 1767},
      year         = {2020},
      abstract     = {Magnesium and calcium chloride salts contribute to the
                      global atmospheric aerosol burden via emission of sea spray
                      and mineral dust. Their influence on aerosol hygroscopicity
                      and cloud forming potential is important but uncertain with
                      ambiguities between results reported in the literature. To
                      address this, we have conducted measurements of the
                      hygroscopic growth and critical supersaturation of dried,
                      size selected nano-particles made from aqueous solution
                      droplets of MgCl2 and CaCl2, respectively, and compare
                      experimentally derived values with results from
                      state-of-the-art thermodynamic modelling. It is
                      characteristic of both MgCl2 and CaCl2 salts that they bind
                      water in the form of hydrates under a range of ambient
                      conditions. We discuss how hydrate formation affects the
                      particles' water uptake and provide an expression for
                      hydrate correction factors needed in calculations of
                      hygroscopic growth factors, critical super-saturations, and
                      derived κ values of particles containing hydrate forming
                      salts. We demonstrate the importance of accounting for
                      hydrate forming salts when predicting hygroscopic properties
                      of sea spray aerosol.},
      cin          = {IEK-8},
      ddc          = {333.7},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {32697206},
      UT           = {WOS:000560533900012},
      doi          = {10.1039/D0EM00179A},
      url          = {https://juser.fz-juelich.de/record/891840},
}