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@ARTICLE{Wang:891842,
      author       = {Wang, Haichao and Chen, Xiaorui and Lu, Keding and Tan,
                      Zhaofeng and Ma, Xuefei and Wu, Zhijun and Li, Xin and Liu,
                      Yuhan and Shang, Dongjie and Wu, Yusheng and Zeng, Limin and
                      Hu, Min and Schmitt, Sebastian and Kiendler-Scharr, Astrid
                      and Wahner, Andreas and Zhang, Yuanhang},
      title        = {{W}intertime {N}2{O}5 uptake coefficients over the {N}orth
                      {C}hina {P}lain},
      journal      = {Science bulletin},
      volume       = {65},
      number       = {9},
      issn         = {2095-9273},
      address      = {[S.l.]},
      publisher    = {Science China Press},
      reportid     = {FZJ-2021-01765},
      pages        = {765 - 774},
      year         = {2020},
      note         = {Kein Post-print vorhanden},
      abstract     = {The heterogeneous hydrolysis of dinitrogen pentoxide (N2O5)
                      plays an important role in regulating NOx. The N2O5 uptake
                      coefficient, γ(N2O5), was determined using an iterative box
                      model that was constrained to observational data obtained in
                      suburban Beijing from February to March 2016. The box model
                      determined 2289 individual γ(N2O5) values that varied from
                      <0.001 to 0.02 with an average value of 0.0046 ± 0.0039
                      (and a median value of 0.0032). We found the derived winter
                      γ(N2O5) values in Beijing were relatively low as compared
                      to values reported in previous field studies conducted
                      during winter in Hong Kong (average value of 0.014) and the
                      eastern U.S. coast (median value of 0.0143). In our study,
                      field evidence of the suppression of γ(N2O5) values due to
                      pNO3− content, organics and the enhancement by aerosol
                      liquid water content (ALWC) is in line with previous
                      laboratory study results. Low ALWC, high pNO3− content,
                      and particle morphology (inorganic core with an organic
                      shell) accounted for the low γ(N2O5) values in the North
                      China Plain (NCP) during wintertime. The field-derived
                      γ(N2O5) values are well reproduced by a revised
                      parameterization method, which includes the aerosol size
                      distribution, ALWC, nitrate and organic coating, suggesting
                      the feasibility of comprehensive parameterization in the NCP
                      during wintertime.},
      cin          = {IEK-8},
      ddc          = {500},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000528833400012},
      doi          = {10.1016/j.scib.2020.02.006},
      url          = {https://juser.fz-juelich.de/record/891842},
}