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000891883 1001_ $$0P:(DE-HGF)0$$aChen, Gong$$b0$$eCorresponding author
000891883 245__ $$aObservation of Hydrogen-Induced Dzyaloshinskii-Moriya Interaction and Reversible Switching of Magnetic Chirality
000891883 260__ $$aCollege Park, Md.$$bAPS$$c2021
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000891883 520__ $$aThe Dzyaloshinskii-Moriya interaction (DMI) has drawn much attention, as it stabilizes magnetic chirality, with important implications in fundamental and applied research. This antisymmetric exchange interaction is induced by the broken inversion symmetry at interfaces or in noncentrosymmetric lattices. Significant interfacial DMIs are often found at magnetic/heavy-metal interfaces with large spin-orbit coupling. Recent studies have shown promise for induced DMI at interfaces involving light elements such as carbon (graphene) or oxygen. Here, we report direct observation of induced DMI by chemisorption of the lightest element, hydrogen, on a ferromagnetic layer at room temperature, which is supported by density functional theory calculations. We further demonstrate a reversible chirality transition of the magnetic domain walls due to the induced DMI via hydrogen chemisorption and desorption. These results shed new light on the understanding of DMI in low atomic number materials and the design of novel chiral spintronics and magneto-ionic devices.
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000891883 7001_ $$00000-0001-5881-8962$$aRobertson, MacCallum$$b1
000891883 7001_ $$0P:(DE-Juel1)162311$$aHoffmann, Markus$$b2
000891883 7001_ $$0P:(DE-HGF)0$$aOphus, Colin$$b3
000891883 7001_ $$00000-0002-0537-7793$$aFernandes Cauduro, André L.$$b4
000891883 7001_ $$00000-0002-5050-9978$$aLo Conte, Roberto$$b5
000891883 7001_ $$00000-0001-7524-0779$$aDing, Haifeng$$b6
000891883 7001_ $$00000-0002-0472-4183$$aWiesendanger, Roland$$b7
000891883 7001_ $$0P:(DE-Juel1)130548$$aBlügel, Stefan$$b8
000891883 7001_ $$00000-0003-0035-3095$$aSchmid, Andreas K.$$b9
000891883 7001_ $$0P:(DE-HGF)0$$aLiu, Kai$$b10$$eCorresponding author
000891883 773__ $$0PERI:(DE-600)2622565-7$$a10.1103/PhysRevX.11.021015$$gVol. 11, no. 2, p. 021015$$n2$$p021015$$tPhysical review / X$$v11$$x2160-3308$$y2021
000891883 8564_ $$uhttps://juser.fz-juelich.de/record/891883/files/PhysRevX.11.021015.pdf$$yOpenAccess
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