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000892391 1001_ $$00000-0003-4420-5609$$aTiso, Till$$b0
000892391 245__ $$aTowards bio-upcycling of polyethylene terephthalate
000892391 260__ $$aOrlando, Fla.$$bAcademic Press$$c2021
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000892391 500__ $$aBiotechnologie 1
000892391 520__ $$aOver 359 million tons of plastics were produced worldwide in 2018, with significant growth expected in the near future, resulting in the global challenge of end-of-life management. The recent identification of enzymes that degrade plastics previously considered non-biodegradable opens up opportunities to steer the plastic recycling industry into the realm of biotechnology.Here, the sequential conversion of post-consumer polyethylene terephthalate (PET) into two types of bioplastics is presented: a medium chain-length polyhydroxyalkanoate (PHA) and a novel bio-based poly(amide urethane) (bio-PU). PET films are hydrolyzed by a thermostable polyester hydrolase yielding highly pure terephthalate and ethylene glycol. The obtained hydrolysate is used directly as a feedstock for a terephthalate-degrading Pseudomonas umsongensis GO16, also evolved to efficiently metabolize ethylene glycol, to produce PHA. The strain is further modified to secrete hydroxyalkanoyloxy-alkanoates (HAAs), which are used as monomers for the chemo-catalytic synthesis of bio-PU. In short, a novel value-chain for PET upcycling is shown that circumvents the costly purification of PET monomers, adding technological flexibility to the global challenge of end-of-life management of plastics.
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000892391 7001_ $$0P:(DE-HGF)0$$aNarancic, Tanja$$b1
000892391 7001_ $$00000-0003-3876-1350$$aWei, Ren$$b2
000892391 7001_ $$00000-0002-4920-7024$$aPollet, Eric$$b3
000892391 7001_ $$0P:(DE-HGF)0$$aBeagan, Niall$$b4
000892391 7001_ $$0P:(DE-HGF)0$$aSchröder, Katja$$b5
000892391 7001_ $$0P:(DE-HGF)0$$aHonak, Annett$$b6
000892391 7001_ $$0P:(DE-HGF)0$$aJiang, Mengying$$b7
000892391 7001_ $$0P:(DE-HGF)0$$aKenny, Shane T.$$b8
000892391 7001_ $$0P:(DE-Juel1)176653$$aWierckx, Nick$$b9
000892391 7001_ $$0P:(DE-HGF)0$$aPerrin, Rémi$$b10
000892391 7001_ $$0P:(DE-HGF)0$$aAvérous, Luc$$b11
000892391 7001_ $$00000-0002-5730-6663$$aZimmermann, Wolfgang$$b12
000892391 7001_ $$0P:(DE-HGF)0$$aO'Connor, Kevin$$b13
000892391 7001_ $$00000-0003-0961-4976$$aBlank, Lars M.$$b14$$eCorresponding author
000892391 773__ $$0PERI:(DE-600)1471017-1$$a10.1016/j.ymben.2021.03.011$$gVol. 66, p. 167 - 178$$p167 - 178$$tMetabolic engineering$$v66$$x1096-7176$$y2021
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